Redox: fundamentals, processes and applications ; with 21 tables
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| Format: | Book |
|---|---|
| Language: | English |
| Published: |
Berlin [u.a.]
Springer
2000
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Item Description: | Literaturangaben |
| Physical Description: | XXI, 251 S. graph. Darst. 24 cm |
| ISBN: | 3540665285 |
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MARC
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| 245 | 1 | 0 | |a Redox |b fundamentals, processes and applications ; with 21 tables |c J. Schüring ... (ed.) |
| 264 | 1 | |a Berlin [u.a.] |b Springer |c 2000 | |
| 300 | |a XXI, 251 S. |b graph. Darst. |c 24 cm | ||
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| adam_text | Contents
Preface.................................................................................................................VII
List of Authors....................................................................................................XIX
Chapter 1
Redox Potential Measurements in Natural Waters: Significance:
Concepts and Problems
LSigg....................................................................................................................../
1.1 Relevance of Redox Potential Measurements.................................................1
1.2 Thermodynamic Definition of Redox Potential..............................................2
1.3 Redox Potential Range in Natural Waters.......................................................5
1.4 Electrochemical Measurement of Redox Potential.........................................6
1.5 Examples of Redox Potential Measurements..................................................8
1.6 Redox Conditions in Natural Waters:
Examples of Lack of Equilibrium.................................................................10
1.7 Conclusions...................................................................................................10
1.8 References.....................................................................................................11
Chapter 2
Technique of Measurement, Electrode Processes and Electrode Treatment
H. Galster..............................................................................................................13
2.1 Electron Transfers.........................................................................................13
2.1.1 Exchange Currents.............................................................................13
Contents_____________________________________________________________XJ
2.1.2 MARCUS-Theory................................................................................15
2.1.3 Practical Rules...................................................................................16
2.2 Electrodes......................................................................................................17
2.2.1 Platinum Electrodes...........................................................................17
2.2.2 Oxygen...............................................................................................18
2.2.3 Mixed Potentials................................................................................19
2.2.4 Pre-Treatment....................................................................................20
2.2.5 Design................................................................................................21
2.2.6 Reference Electrodes.........................................................................22
2.3 References.....................................................................................................23
Chapter 3
Characterisation of the Redox State of Aqueous Systems:
Towards a Problem-Oriented Approach
S.Peiffer................................................................................................................24
3.1 Introduction...................................................................................................24
3.2 pHandpe......................................................,...............................................25
3.3 Measurement of Redox Voltages at Redox Electrodes.................................27
3.4 New Perspectives..........................................................................................30
3.4.1 Hydrogen Concentration as a Master Variable to Characterise
Metabolic Organic Matter Degradation.............................................31
3.4.2 The Partial Equilibrium Approach.....................................................33
3.4.3 The Use of the pH2S-Value to Quantify the Redox State
of Sulfidic Systems............................................................................34
3.4.4 The Use of Probe Compounds to Characterise the Reactivity
of a Solution.......................................................................................37
3.5 Summary and Conclusion.............................................................................38
3.6 References.....................................................................................................39
Chapter 4
Comparison of Different Methods for Redox Potential Determination
in Natural Waters
M.Kolling..............................................................................................................42
4.1 Introduction...................................................................................................42
4.2 Redox Potential Calculations........................................................................43
4.2.1 The H2O/O2-Couple...........................................................................44
4.2.2 Fe-Species..........................................................................................45
4.2.3 As-Species.........................................................................................45
4.2.4 S-Species............................................................................................46
4.2.5 N-Species...........................................................................................46
4.2.6 The CO2/CH4-CoupIe.........................................................................47
XII_______________________________________________________Contents
4.3 Redox Potential Measurements.....................................................................47
4.3.1 Metal Electrodes................................................................................48
4.3.2 Reference Electrodes.........................................................................48
4.3.3 Calibration Solutions.........................................................................48
4.4 Material and Methods...................................................................................49
4.4.1 The Artesian Well Schierensee .......................................................49
4.4.2 Electrodes..........................................................................................49
4.4.3 Instruments.........................................................................................50
4.5 Results...........................................................................................................50
4.5.1 Redox Potential Measurements..........................................................50
4.5.2 Calculation of Redox Potentials.........................................................51
4.6 Discussion.....................................................................................................52
4.6.1 Redox Potential Measurements..........................................................52
4.6.2 Redox Potential Calculations.............................................................53
4.7 Conclusions...................................................................................................53
4.8 References.....................................................................................................53
Chapter 5
A Novel Approach to the Presentation of pe/pH-Diagrams
M. Kolling, M. Ebert H.D. Schulz......................................................................55
5.1 Introduction...................................................................................................55
5.2 Construction of pe/pH-Diagrams..................................................................56
5.3 Disadvantages of Classical pe/pH-Diagrams................................................60
5.4 New Presentation of pe/pH-Diagrams...........................................................60
5.5 Conclusions...................................................................................................63
5.6 References.....................................................................................................63
Chapter 6
The Couple As(V) - As(III) as a Redox Indicator
T.R.Rude S. Wohnlich.......................................................................................64
6.1 Introduction...................................................................................................64
6.2 The Procedure...............................................................................................65
6.2.1 Sampling............................................................................................66
6.2.2 Analysis.............................................................................................67
6.2.3 Analysing the Major Ions...................................................................69
6.2.4 Calculating the Ion Strength..............................................................70
6.2.5 Calculating the Activity Coefficients.................................................71
6.2.6 Calculating the Activities of the As-Species......................................72
6.2.7 Drawing up a System of Thermodynamic Redox Equations.............74
6.2.8 Solving the Thermodynamic Equations to get pe..............................77
6.3 Conclusions...................................................................................................77
Contents______________________________________________________XIII
6.4 Acknowledgements.......................................................................................78
6.5 References.....................................................................................................78
Chapter 7
In Situ Long-Term-Measurement of Redox Potential in Redoximorphic Soils
S. Fiedler...............................................................................................................81
7.1 Introduction...................................................................................................81
7.2 Study Sites and Soils.....................................................................................82
7.3 Methods.........................................................................................................83
7.3.1 Redox Measurements.........................................................................83
7.3.2 Methane Measurements.....................................................................84
7.3.3 Spatial and Temporal Variability of EH.............................................85
7.4 Reasons for EH-Variations in Soils................................................................88
7.4.1 Temperature.......................................................................................88
7.4.2 Water Regime....................................................................................89
7.4.2.1 Precipitation.........................................................................89
7.4.2.2 Groundwater........................................................................91
7.5 Relationship Between Redox Conditions and Methane Flux........................92
7.6 Conclusion....................................................................................................93
7.7 References.....................................................................................................93
Chapter 8
Redox Measurements as a Qualitative Indicator of Spatial and
Temporal Variability of Redox State in a Sandy Forest Soil
A. Teichert.J. Bottcher W.H.M. Duijnisveld.....................................................95
8.1 Introduction...................................................................................................95
8.2 Material and Methods...................................................................................97
8.2.1 Investigation Site...............................................................................97
8.2.2 Transect Measurements.....................................................................98
8.2.3 Electrodes..........................................................................................99
8.2.4 EH-and pe-Values..............................................................................99
8.2.5 Statistical Data Analysis..................................................................100
8.3 Results and Discussion................................................................................101
8.3.1 EH and pH at a Depth of 0.8 m and of 1.1 m....................................101
8.3.2 EH at a Depth of 1.4 m.....................................................................102
8.4 Conclusions.................................................................................................108
8.5 References...................................................................................................109
XIV_______________________________________________________Contents
Chapter 9
Implementation of Redox Reactions in Groundwater Models
W. Schafer............................................................................................................///
9.1 Introduction.................................................................................................Ill
9.2 The Redox Potential as Controlling Variable..............................................112
9.2.1 Equilibrium Models.........................................................................112
9.2.2 Combined Approach........................................................................114
9.3 Models that do not Explicitly Consider the Redox Potential......................115
9.3.1 Superposition Models......................................................................115
9.3.2 Kinetic Models with Specified Reaction Rate Constants.................116
9.3.3 Models with Variable Kinetics........................................................117
9.4 Summary.....................................................................................................118
9.5 References...................................................................................................119
Chapter 10
Variance of the Redox Potential Value in Two Anoxic Groundwater Systems
M. Kofod..............................................................................................................120
10.1 Introduction..............................................................................................120
10.2 Groundwater in the River Marsh of the Elbe (Hamburg).........................121
10.2.1 Variation of the Measured EH-Values........................................122
10.2.2 Spatial Distribution....................................................................124
10.2.3 Correlation Between the EH-Value and the
Chemical Composition of the Groundwater...............................124
10.3 Groundwater in the Oderbruch (Brandenburg).........................................127
10.3.1 Variation of the Measured Eh-Values........................................128
10.3.2 Spatial Distribution....................................................................129
10.3.3 Correlation Between the EH-Value and the
Chemical Composition of the Groundwater...............................130
10.4 Interpretation and Conclusion..................................................................132
10.5 Acknowledgements..................................................................................134
10.6 References................................................................................................134
Chapter 11
Redox Fronts in Aquifer Systems and Parameters Controlling their Dimensions
J. Schiiring, M. Schlieker J. Hencke................................................................135
11.1 Introduction ...........................................................................................135
11.2 Regional Scales of Redox Fronts in Aquifer Systems..............................137
11.3 Investigating the Scales of Redox Fronts.................................................139
11.3.1 Column Tests..............................................................................139
Contents XV
11.3.1.1 Flow Rate versus Decomposition Rate......................141
11.3.2 Lake Sediments..........................................................................143
11.3.3 Bank Infiltration.........................................................................147
11.4 Summary.................................................................................................149
11.5 References ...........................................................................................150
Chapter 12
Redox Processes Active in Denitrification
C.G.E.M. vanBeek..............................................................................................152
12.1 Introduction..............................................................................................152
12.2 Site and Methods......................................................................................153
12.3 Geochemistry...........................................................................................153
12.3.1 Denitrification............................................................................155
12.3.2 Reduction Capacity....................................................................157
12.4 Conclusions..............................................................................................159
12.5 Acknowledgement....................................................................................159
12.6 References................................................................................................160
Chapter 13
Measurement of Redox Potentials at the Test Site Insel Hengsen
U. Schulte-Ebbert T. Hofmann........................................................................161
13.1 Introduction..............................................................................................161
13.2 The Test Site.............................................................................................162
13.3 Observed Redox Conditions.....................................................................163
13.4 Interpretation Problems............................................................................165
13.5 Groundwater Sampling and Redox Measurement....................................167
13.6 Kinetics of Redox Measurements.............................................................169
13.7 Conclusions and Recommendations.........................................................172
13.8 Acknowledgements..................................................................................173
13.9 References................................................................................................173
Chapter 14
Redox Reactions, Multi-Component Stability Diagrams and Isotopic
Investigations in Sulfur- and Iron-Dominated Groundwater Systems
F. Wisotzky..........................................................................................................175
14.1 Introduction..............................................................................................175
XVI Contents
14.2 Methods....................................................................................................176
14.2.1 Locations of the Study Area.......................................................176
14.2.2 Sediment and Water Analyses....................................................176
14.2.3 Analysis of Isotopes...................................................................177
14.2.4 Multi-Component Stability Diagrams (pH-pe-Diagrams)..........177
14.3 Results......................................................................................................178
14.3.1 Mobilising Reactions of Sulfur and Iron....................................178
14.3.2 Immobilising Reactions of Sulfur and Iron................................181
14.4 Summary..................................................................................................186
14.5 References................................................................................................187
Chapter 15
Redox Buffer Capacity Concept as a Tool for the Assessment of Long-Term
Effects in Natural Attenuation / Intrinsic Remediation
F. von der Kammer, J. Thoming U. Forstner..................................................189
15.1 Introduction..............................................................................................189
15.1.1 Natural Attenuation....................................................................189
15.1.1.1 Redox Processes in the Natural Attenuation
Concept......................................................................190
15.1.1.2 Practical Experience and Priority Parameters............191
15.1.2 Contaminant Plumes in Groundwater........................................192
15.1.3 Redox Buffer Capacity...............................................................193
15.2 Redox Buffer Capacities: Conceptional Approach...................................194
15.3 Analytical Approach and Application......................................................195
15.3.1 Overview....................................................................................195
15.3.1.1 OXC..........................................................................195
15.3.1.2 TRC...........................................................................196
15.3.2 Case Study:
Simplified Illustration of a Groundwater Plume s Redox
Activities by Common Sequential Extraction............................196
15.3.2.1 Determination of the Total Reduction Capacity
(TRC)........................................................................196
15.3.2.2 Soil Sample and Extraction Scheme..........................197
15.3.2.3 Results and Discussion of the Case Study.................198
15.4 Conclusions..............................................................................................200
15.5 References................................................................................................201
Contents XVII
Chapter 16
Redox Zones in the Plume of a Previously Operating Gas Plant
K. Weber, N. Brandsch, B. Reichert, M. Eiswirth, H. Hotzl,
O. Hummer A. Dahmke....................................................................................203
16.1 Introduction..............................................................................................203
16.2 Geology and Hydrology...........................................................................205
16.3 Methods and Materials.............................................................................207
16.4 Results and Discussion.............................................................................208
16.5 Summary and Conclusions.......................................................................215
16.6 References................................................................................................215
Chapter 17
Degradation of Organic Groundwater Contaminants:
Redox Processes and EH-Values
M. Ebert, O. Hummer, M. Mayer, O. Schlicker A. Dahmke............................217
17.1 Introduction..............................................................................................217
17.2 Degradation of BTX in the Underground of a Former Gas Plant.............219
17.3 Reductive Dehalogenation of Chlorinated Hydrocarbons........................222
17.4 Conclusions..............................................................................................225
17.5 References................................................................................................226
Chapter 18
Microbial Metabolism of Iron Species in Freshwater Lake Sediments
B.Schink M. Bern............................................................................................228
18.1 Introduction..............................................................................................228
18.2 Iron Compounds in Lake Constance Sediments.......................................230
18.3 Microbial Oxidation of Iron Compounds.................................................231
18.4 Reduction of Ferric Iron Hydroxides........................................................232
18.5 Conclusions..............................................................................................233
18.6 Acknowledgements..................................................................................234
18.7 References................................................................................................234
XVIII___________________________________________________________Contents
Chapter 19
Redox Measurements in Marine Sediments
H.D.Schulz..........................................................................................................235
19.1 The Scope of Redox Measurements.........................................................235
19.2 How Measurements are Performed..........................................................238
19.3 Typical EH-Profiles and their Interpretation.............................................239
19.4 Precision and Reproducibility..................................................................243
19.5 Relevance of the Results..........................................................................245
19.6 References................................................................................................246
* * *
Subject Index.......................................................................................................248
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| genre | (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV012884852 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:35:28Z |
| institution | BVB |
| isbn | 3540665285 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-008771064 |
| oclc_num | 247850372 |
| open_access_boolean | |
| owner | DE-703 DE-12 DE-739 DE-29 DE-M49 DE-BY-TUM DE-634 DE-83 DE-11 DE-188 |
| owner_facet | DE-703 DE-12 DE-739 DE-29 DE-M49 DE-BY-TUM DE-634 DE-83 DE-11 DE-188 |
| physical | XXI, 251 S. graph. Darst. 24 cm |
| publishDate | 2000 |
| publishDateSearch | 2000 |
| publishDateSort | 2000 |
| publisher | Springer |
| record_format | marc |
| spelling | Redox fundamentals, processes and applications ; with 21 tables J. Schüring ... (ed.) Berlin [u.a.] Springer 2000 XXI, 251 S. graph. Darst. 24 cm txt rdacontent n rdamedia nc rdacarrier Literaturangaben Umweltgeochemie - Redoxreaktion - Aufsatzsammlung Environmental geochemistry Oxidation-reduction reaction Ökologische Chemie (DE-588)4135167-8 gnd rswk-swf Redoxreaktion (DE-588)4177303-2 gnd rswk-swf Geochemie (DE-588)4020198-3 gnd rswk-swf Umweltgeochemie (DE-588)4404136-6 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Redoxreaktion (DE-588)4177303-2 s DE-604 Ökologische Chemie (DE-588)4135167-8 s Geochemie (DE-588)4020198-3 s Umweltgeochemie (DE-588)4404136-6 s DE-188 Schüring, Joachim Sonstige oth HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008771064&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Redox fundamentals, processes and applications ; with 21 tables Umweltgeochemie - Redoxreaktion - Aufsatzsammlung Environmental geochemistry Oxidation-reduction reaction Ökologische Chemie (DE-588)4135167-8 gnd Redoxreaktion (DE-588)4177303-2 gnd Geochemie (DE-588)4020198-3 gnd Umweltgeochemie (DE-588)4404136-6 gnd |
| subject_GND | (DE-588)4135167-8 (DE-588)4177303-2 (DE-588)4020198-3 (DE-588)4404136-6 (DE-588)4143413-4 |
| title | Redox fundamentals, processes and applications ; with 21 tables |
| title_auth | Redox fundamentals, processes and applications ; with 21 tables |
| title_exact_search | Redox fundamentals, processes and applications ; with 21 tables |
| title_full | Redox fundamentals, processes and applications ; with 21 tables J. Schüring ... (ed.) |
| title_fullStr | Redox fundamentals, processes and applications ; with 21 tables J. Schüring ... (ed.) |
| title_full_unstemmed | Redox fundamentals, processes and applications ; with 21 tables J. Schüring ... (ed.) |
| title_short | Redox |
| title_sort | redox fundamentals processes and applications with 21 tables |
| title_sub | fundamentals, processes and applications ; with 21 tables |
| topic | Umweltgeochemie - Redoxreaktion - Aufsatzsammlung Environmental geochemistry Oxidation-reduction reaction Ökologische Chemie (DE-588)4135167-8 gnd Redoxreaktion (DE-588)4177303-2 gnd Geochemie (DE-588)4020198-3 gnd Umweltgeochemie (DE-588)4404136-6 gnd |
| topic_facet | Umweltgeochemie - Redoxreaktion - Aufsatzsammlung Environmental geochemistry Oxidation-reduction reaction Ökologische Chemie Redoxreaktion Geochemie Umweltgeochemie Aufsatzsammlung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008771064&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT schuringjoachim redoxfundamentalsprocessesandapplicationswith21tables |