Introduction to ionomers:
Saved in:
| Main Authors: | , |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
New York [u.a.]
Wiley
1998
|
| Series: | A Wiley-Interscience publication
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XXI, 327 S. Ill., graph. Darst. |
| ISBN: | 0471246786 |
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| adam_text | INTRODUCTION TO IONOMERS ADI EISENBERG DEPARTMENT OF CHEMISTRY MCGILL
UNIVERSITY MONTREAL, QUEBEC, CANADA JOON-SEOP KIM DEPARTMENT OF
CHEMISTRY MCGILL UNIVERSITY MONTREAL, QUEBEC, CANADA & DEPARTMENT OF
POLYMER SCIENCE & ENGINEERING CHOSUN UNIVERSITY KWANGJU, KOREA A
WILEY-LNTERSCIENCE PUBLICATION JOHN WILEY & SONS, INC. NEW YORK /
CHICHESTER / WEINHEIM / BRISBANE / SINGAPORE / TORONTO CONTENTS PREFACE
XIII LIST OF SYMBOLS AND ABBREVIATIONS XV 1 INTRODUCTION 1 1.1.
DEFINITIONS / 2 1.2. NOMENCLATURE / 3 1.3. HISTORICAL ASPECTS / 4 1.4.
REASONS FOR INTEREST IN IONOMERS / 7 1.5. AIMS OF THE PRESENTATION / 8
1.6. IONIC INTERACTIONS / 9 1.7. SIZES OF IONIC GROUPS / 9 1.8. METHODS
OF EXPRESSING ION CONCENTRATIONS /11 1.9. TOPICS OMITTED FROM THIS
TREATMENT / 12 1.10. ORDER OF PRESENTATION /12 1.11. REFERENCES /13 2
STRUCTURAL VARIABILITY IN LONOMERS 17 2.1. ARCHITECTURAL VARIATION / 17
2.1.1. MONOCHELICS, TELECHELICS, AND BLOCK COPOLYMERS / 17 2.1.1.1.
SINGLE IONS AT CHAIN ENDS I 17 2.1.1.2. TELECHELICS I 19 V VI CONTENTS
2.1.1.3. BLOCK COPOLYMERS I 20 2.1.2. SIMPLE RANDOM COPOLYMERS / 23
2.1.3. OTHER IONOMER FAMILIES / 25 2.1.3.1. CHAINS WITH REGULARLY SPACED
IONS I 25 2.1.3.2. COMBS I 25 2.1.3.3. GRAFTS I 28 2.1.3.4. POLYMER-SALT
MIXTURES I 28 2.2. CHEMICAL STRUCTURES / 28 2.2.1. TYPE OF ATTACHMENT OF
PENDENT ION / 28 2.2.2. NATURE OF PENDENT IONS / 29 2.2.3. COUNTERIONS /
30 2.2.4. THE NONIONIC HOST POLYMER / 32 2.2.5. INORGANIC SYSTEMS / 33
2.3. CONCLUDING COMMENTS / 34 2.4. REFERENCES / 34 3 MORPHOLOGY OF
RANDOM LONOMERS 38 3.1. MULTIPLETS / 38 3.1.1. SIZE AND SHAPE OF
MULTIPLET / 38 3.1.1.1. ENERGETICS I 38 3.1.1.2. SOLID ANGLE AND CONTACT
SURFACE AREA CONCEPTS I 39 3.1.1.3. SHAPES OF MULTIPLETS I 39 3.1.1.4.
EFFECT OF ION CONTENT AND DIELECTRIC CONSTANT I 40 3.1.1.5. OTHER
FACTORS I 40 3.1.2. ARRANGEMENTS OF ION PAIRS / 40 3.1.3. ARRANGEMENT OF
THE MULTIPLETS / 41 3.1.3.1. SMALL-ANGLE IONIC PEAK I 41 3.1.3.2.
MULTIPLET-CLUSTER CONCEPT I 42 3.1.3.3. HARD-SPHERE MODEL I 42 3.1.3.4.
CORE-SHELL MODEL I 42 3.1.3.5. DILEMMA OF HARD-SPHERE AND CORE-SHELL
MODELS I 43 3.1.3.6. MORPHOLOGICAL CONTINUITY AND MECHANICAL PROPERTIES
I 44 3.2. EHM MODEL / 45 3.2.1. RESTRICTED MOBILITY REGION / 45 3.2.2.
NEW CLUSTER CONCEPT / 47 3.2.3. PREVALENT INTERMULTIPLET DISTANCE / 49
3.2.4. SEMIQUANTITATIVE ASPECTS / 49 CONTENTS VII 3.3. EXPERIMENTAL
CORROBORATION / 50 3.3.1. SMALL-ANGLE X-RAY SCATTERING PEAK / 50 3.3.2.
DYNAMIC MECHANICAL STUDIES /51 3.3.3. VOLUME FRACTION OF CLUSTERS / 52
3.3.4. THICKNESS OF THE RESTRICTED MOBILITY LAYER / 52 3.3.5.
UNCLUSTERED MATERIALS AND HOMOBLENDS / 53 3.3.6. EXPERIMENTAL EVIDENCE
FOR REDUCED MOBILITY / 53 3.4. COIL DIMENSIONS IN RANDOM IONOMERS / 54
3.5. REFERENCES / 55 4 GLASS TRANSITIONS IN RANDOM IONOMERS 59 4.1.
EFFECT OF IONIC FORCES / 59 4.2. GLASS TRANSITION VERSUS ELECTROSTATIC
WORK / 61 4.3. TWO GLASS TRANSITIONS / 62 4.3.1. TWO LOSS TANGENT PEAKS
/ 63 4.3.2. TWO GLASS TRANSITIONS BY DSC / 63 4.3.3. EXPANSION
COEFFICIENTS / 65 4.4. MATRIX GLASS TRANSITION / 65 4.4.1. THE
CHARGE/DISTANCE EFFECT / 65 4.4.2. GLASS TRANSITION VERSUS PERCENT
NEUTRALIZATION / 69 4.4.3. COPOLYMERIZATION, CROSS-LINKING, AND FILLER
EFFECTS / 69 4.4.4. CHANGE IN GLASS TRANSITION AS A FUNCTION OF CHANGE
IN ION CONCENTRATION /71 4.4.5. AMMONIUM COUNTERIONS / 72 4.4.6.
INTERNAL PLASTICIZATION EFFECT / 73 4.4.7. SEMICRYSTALLINE MATERIALS /
74 4.4.8. THEORIES / 74 4.5. CLUSTER GLASS TRANSITION / 75 4.5.1. EFFECT
OF IMMOBILIZATION / 75 4.5.2. DIFFERENCES IN THE TWO GLASS TRANSITION
TEMPERATURE VALUES / 77 4.5.3. HOMOBLENDS / 79 4.5.4. UNCLUSTERED
MATERIALS / 81 4.5.5. DIFFERENCES IN CLUSTERING BEHAVIOR OF STYRENE
IONOMERS / 81 4.5.6. MECHANISM OF THE CLUSTER GLASS TRANSITION / 82 4.6.
REFERENCES / 83 VIII CONTENTS 5 STYRENE IONOMERS 86 5.1.
STRESS-RELAXATION OF SODIUM METHACRYLATE SYSTEMS / 87 5.2. DYNAMIC
MECHANICAL STUDIES OF SODIUM METHACRYLATE SYSTEMS / 89 5.2.1. GLASSY
MODULUS / 89 5.2.2. LOSS TANGENT PEAKS / 89 5.2.3. IONIC MODULUS / 90
5.2.4. CROSS-LINKING / 90 5.2.5. FILLER / 92 5.2.6. PERCOLATION / 94
5.3. MELT RHEOLOGY OF SODIUM METHACRYLATE SYSTEMS / 95 5.4.
VISCOELASTICITY OF OTHER CARBOXYLATED IONOMERS / 96 5.4.1. P(S-CO-ANA)
VERSUS P(S-CO-MANA) / 98 5.4.2. P(S-CO-SCNA) VERSUS P(S-CO-MANA) / 98
5.4.3. COMBS / 99 5.5. PENDENT ION EFFECT ON VISCOELASTICITY / 101
5.5.1. SULFONATED IONOMERS / 101 5.5.2. BENZYLOXY OR PHENOXY IONOMERS /
104 5.5.3. VINYLPYRIDINIUM METHYL IODIDE IONOMERS / 105 5.5.4.
HOMOBLENDS / 106 5.6. EFFECTS OF VARIOUS OTHER PARAMETERS / 109 5.6.1.
DIELECTRIC CONSTANT / 109 5.6.2. COUNTERIONS /110 5.6.3. MOLECULAR
WEIGHT / 111 5.6.4. DEGREE OF NEUTRALIZATION /111 5.7. ION HOPPING /114
5.8. OTHER PHYSICAL PROPERTIES AND SPECTROSCOPY / 117 5.8.1. DENSITY /
117 5.8.2. DIELECTRIC PROPERTIES / 118 5.8.3. SPECTROSCOPY / 122
5.8.3.1. INFRARED I 122 5.8.3.2. RAMAN I 125 5.8.3.3. NUCLEAR MAGNETIC
RESONANCE I 125 5.8.3.4. ELECTRON SPIN RESONANCE I 126 5.8.3.5. EXTENDED
X-RAY ABSORPTION FINE STRUCTURE I 127 5.8.4. ORIENTATION / 129 5.8.5.
GAS TRANSPORT / 131 5.8.6. WATER ABSORPTION / 132 5.8.7. TRANSPORT OF
NONGASEOUS MATERIALS / 133 CONTENTS 5.9. FATIGUE AND FRACTURE PROPERTIES
/ 136 5.10. NONEQUILIBRIUM BEHAVIOR / 137 5.11. CHEMISTRY IN IONOMERS /
141 5.11.1. STABILITY / 141 5.11.2. REACTIONS IN IONOMERS / 143 5.12.
REFERENCES / 143 6 PARTLY CRYSTALLINE IONOMERS 6.1. POLYETHYLENE / 150
6.2. 6.3. 6.1.1. 6.1.2. 6.1.3. 6.1.4. 6.1.5. 6.1.6. 6.1.7. 6.1.8. 6.1.9.
6.1.10. 6.1.11. STRESS-RELAXATION / 150 DYNAMIC MECHANICAL PROPERTIES /
151 MELT RHEOLOGY / 152 OTHER MECHANICAL PROPERTIES / 153 DIELECTRIC
PROPERTIES / 153 SPECTROSCOPY / 156 6.1.6.1. INFRARED 1 156 6.1.6.2.
RAMAN 1 158 6.1.6.3. ELECTRON SPIN RESONANCE 1 158 6.1.6.4. NUCLEAR
MAGNETIC RESONANCE 1 159 WATER UPTAKE / 160 CRYSTALLINITY / 160
PERMEATION / 162 ORIENTATION / 163 CONCLUDING COMMENTS /164
POLYTETRAFLUOROETHYLENE /164 6.2.1. 6.2.2. 6.2.3. 6.2.4. 6.2.5. 6.2.6.
6.2.7. 6.2.9. 6.2.10. CRYSTALLINITY / 165 MECHANICAL PROPERTIES / 166
OTHER PHYSICAL PROPERTIES / 169 DIELECTRIC PROPERTIES / 171 SPECTROSCOPY
/172 6.2.5.1. NUCLEAR MAGNETIC RESONANCE 1 172 6.2.5.2. INFRARED 1 172
MORPHOLOGY / 173 WATER UPTAKE AND DIFFUSION / 175 PERMEATION /179
CHEMISTRY / 182 POLYPENTENAMER / 183 6.3.1. 6.3.2. 6.3.3. SYNTHESIS AND
THERMAL PROPERTIES / 183 MECHANICAL PROPERTIES /183 MORPHOLOGY / 184
CONTENTS 6.4. REFERENCES / 184 OTHER IONOMERS 190 7.1. IONOMERS WITH
STATISTICAL ION PLACEMENT / 190 7.1.1. ELASTOMERS / 190 7.1.1.1.
BUTADIENE-BASED ELASTOMERS I 190 7.1.1.2. ETHYLENE-PROPYLENE-DIENE
TERPOLYMERS I 192 7.1.1.3. POLYURETHANE IONOMERS I 193 7.1.3.1.1.
PHYSICAL PROPERTIES I 194 7.1.1.3.2. MORPHOLOGY I 202 7.1.2. ACRYLATE
AND METHACRYLATE IONOMERS / 204 7.1.3. ZWITTERIONIC SYSTEMS / 209
7.1.3.1. SILOXANE-BASED DI-ZWITTERIONOMERS I 209 7.1.3.2.
HYDROCARBON-BASED ZWITTERIONOMERS I 210 7.2. IONOMERS WITH REGULAR
ARCHITECTURES / 214 7.2.1. BLOCK IONOMERS / 214 7.2.1.1. MORPHOLOGY I
214 7.2.1.2. MECHANICAL PROPERTIES I 218 7.2.2. MONOCHELICS,
TELECHELICS, AND STARS / 220 7.2.2.1. MONOCHELICS I 221 7.2.2.2.
TELECHELICS I 221 7.2.2.3. STARS I 224 7.2.3. IONENES / 229 7.2.4.
POLYMER-SALT MIXTURES / 233 7.3. REFERENCES / 238 PLASTICIZATION 244
8.1. SMALL MOLECULE PLASTICIZERS OF HIGH POLARITY / 245 8.1.1.
MECHANICAL PROPERTIES / 245 8.1.2. MORPHOLOGY / 248 8.2. PLASTICIZERS OF
LOW POLARITY / 250 8.2.1. SMALL MOLECULE PLASTICIZERS / 250 8.2.1.1.
MECHANICAL PROPERTIES I 250 8.2.1.2. MORPHOLOGY I 254 8.2.2. OLIGOMERIC
PLASTICIZERS / 255 8.3. AMPHIPHILIC PLASTICIZERS / 256 8.3.1.
SURFACTANTS / 256 8.3.2. OLIGOMERIC AMPHIPHILES / 258 CONTENTS XI
8.3.2.1. MECHANICAL PROPERTIES I 258 8.3.2.2. MORPHOLOGY I 260 8.3.3.
AMINES / 261 8.4. INTERNAL PLASTICIZATION / 262 8.4.1. MECHANICAL
PROPERTIES / 262 8.4.2. MORPHOLOGY / 263 8.5. SUMMARY / 264 8.6.
REFERENCES / 265 9 IONOMER BLENDS 267 9.1. TECHNIQUES FOR CHARACTERIZING
MISCIBILITY / 268 9.2. MENU OF INTERACTIONS / 269 9.3. MORPHOLOGY / 272
9.4. CROSS-LINKING AND PLASTICIZATION / 272 9.5. ION-ION BLENDS / 274
9.6. ION PAIR-ION PAIR BLENDS / 280 9.7. ION-DIPOLE BLENDS / 282 9.8.
ION-COORDINATION BLENDS / 289 9.9. MISCELLANEOUS BLENDS / 296 9.9.1.
TELECHELIC BLENDS / 296 9.9.2. BLENDS OF LONOMERS WITH THEIR NONIONIC
PARENT POLYMERS / 299 9.9.3. STYRENE IONOMER-POLY(PHENYLENE OXIDE)
BLENDS / 301 9.10. CONCLUDING REMARKS / 302 9.11. REFERENCES / 302 10
APPLICATIONS 307 10.1. MEMBRANES AND THIN FILMS / 307 10.1.1. MEMBRANES
/ 307 10.1.2. PACKAGING / 308 10.1.3. FERTILIZER / 309 10.1.4. FLOOR
POLISH / 309 10.1.5. IMAGING SYSTEMS /310 10.1.6. MAGNETIC RECORDING
MEDIA /311 10.1.7. ADHESIVES /311 10.2. LONOMERS IN BULK / 311 10.2.1.
PLASTICS /311 10.2.2. ELASTOMERS /312 XII CONTENTS 10.3. DRILLING FLUIDS
/ 312 10.4. CATALYSTS AND CATALYTIC SUPPORTS /312 10.5. REFERENCES /313
INDEX 315
|
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| indexdate | 2024-07-09T18:21:55Z |
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| physical | XXI, 327 S. Ill., graph. Darst. |
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| spelling | Eisenberg, Adi Verfasser aut Introduction to ionomers Adi Eisenberg ; Joon-Seop Kim New York [u.a.] Wiley 1998 XXI, 327 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier A Wiley-Interscience publication Ionomeren gtt Ionomères Ionomères ram Ions ram Polymères ram Ionomers Ionomere (DE-588)4162375-7 gnd rswk-swf Ionomere (DE-588)4162375-7 s DE-604 Kim, Joon-Seop Verfasser aut GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008202885&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Eisenberg, Adi Kim, Joon-Seop Introduction to ionomers Ionomeren gtt Ionomères Ionomères ram Ions ram Polymères ram Ionomers Ionomere (DE-588)4162375-7 gnd |
| subject_GND | (DE-588)4162375-7 |
| title | Introduction to ionomers |
| title_auth | Introduction to ionomers |
| title_exact_search | Introduction to ionomers |
| title_full | Introduction to ionomers Adi Eisenberg ; Joon-Seop Kim |
| title_fullStr | Introduction to ionomers Adi Eisenberg ; Joon-Seop Kim |
| title_full_unstemmed | Introduction to ionomers Adi Eisenberg ; Joon-Seop Kim |
| title_short | Introduction to ionomers |
| title_sort | introduction to ionomers |
| topic | Ionomeren gtt Ionomères Ionomères ram Ions ram Polymères ram Ionomers Ionomere (DE-588)4162375-7 gnd |
| topic_facet | Ionomeren Ionomères Ions Polymères Ionomers Ionomere |
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