Microcanonical phase transitions: fragmentation and Coulomb explosion of metal clusters
Saved in:
| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | German |
| Published: |
Berlin
Wiss.-und-Technik-Verl.
1997
|
| Edition: | 1. Aufl. |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | 148 S. Ill., graph. Darst. |
| ISBN: | 3896854275 |
Staff View
MARC
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| 100 | 1 | |a Schapiro, Olga |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Microcanonical phase transitions |b fragmentation and Coulomb explosion of metal clusters |c Olga Schapiro |
| 250 | |a 1. Aufl. | ||
| 264 | 1 | |a Berlin |b Wiss.-und-Technik-Verl. |c 1997 | |
| 300 | |a 148 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 502 | |a Zugl.: Berlin, Freie Univ., Diss., 1997 | ||
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Record in the Search Index
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| adam_text |
CONTENTS
1
INTRODUCTION:
STATISTICS
VERSUS
DYNAMICS
11
1.1
STATISTICAL
PICTURE
.
13
1.1.1
MICROCANONICAL
THERMODYNAMICS
.
14
1.1.2
WHY
NOT
THE
CANONICAL
OR
THE
GRAND
CANONICAL
ENSEMBLE?
.
16
1.2
WHAT
ARE
PHASE
TRANSITIONS
IN
A
FINITE
SYSTEM?
INFLUENCE
OF
CONSERVATION
LAWS
.
19
1.3
THE
TARGET
OF
THIS
WORK
.
22
2
MICROCANONICAL
PHASE
TRANSITIONS
23
2.1
NEGATIVE
TEMPERATURES:
AN
EXAMPLE
OF
AN
IDEAL
PARAMAGNETIC
CRYSTAL
23
2.2
A
PRIMITIVE
MODEL
OF
FRAGMENTATION
.
25
2.2.1
PARTITION
ENTROPY
.
26
2.2.2
DYNAMICAL
ENTROPY
.
26
2.2.3
FRAGMENTATION
PHASE
TRANSITION
.
28
2.3
FIRST
ORDER
PHASE
TRANSITION
IN
THE
POTTS
MODEL
.
34
3
FISSION
AND
FRAGMENTATION
OF
METALLIC
CLUSTERS
39
3.1
SHELL
STRUCTURE
OF
CLUSTERS
.
39
3.2
CLUSTER
STABILITY
.
41
3.2.1
LIQUID
DROP
MODEL
.
41
3.2.2
EVAPORATION
RATE
.
41
3.2.3
CRITICAL
SIZES
.
42
3.3
EXPERIMENTAL
TECHNIQUES
.
42
3.4
A
SHORT
THEORETICAL
OVERVIEW
.
43
3.4.1
MOLECULAR
DYNAMICS
AGAINST
MONTE
CARLO
SIMULATIONS
.
43
3.5
PHASE
TRANSITIONS
IN
CLUSTERS
.
44
8
CONTENTS
4
MMMC
MODEL
IN
APPLICATION
TO
ATOMIC
CLUSTERS
45
4.1
AIM OF
THE
MODEL
.
45
4.2
SIMULATION
METHOD
.
47
4.2.1
MICROCANONICAL
METROPOLIS
MONTE
CARLO
.
48
4.2.2
CONSERVATION
LAWS
.
49
4.2.3
MASSES
AND
CHARGES
OF
THE
FRAGMENTS
.
50
4.2.4
MAXIMAL
EXCITATION
ENERGY
OF
THE
OUTCOMING
FRAGMENTS
.
51
4.2.5
MANY-BODY
POLARIZATION
EFFECTS
.
52
4.3
ASSUMPTIONS
OF
THE
MODEL
.
53
4.3.1
DOMAIN
OF
APPLICABILITY
.
53
5
FRAGMENTATION
PHASE
TRANSITIONS
57
5.1
PHASE
TRANSITIONS
IN
NAJJ
DECAY
.
57
5.2
INCREASING
THE
MASS
OF
THE
NA
2+
CLUSTER
.
62
5.3
NA
5+
FRAGMENTATION
.
62
5.4
EVOLUTION
OF
PHASE
TRANSITION
WITH
RAISING
MASS
OF
THE
MOTHER
CLUSTER.
65
5.5
MATERIAL
DEPENDENCE
OF
THE
TRANSITION
.
67
5.5.1
ALKALI
METAL
CLUSTERS
.
68
5.5.2
ANTIMONY
CLUSTERS
.
70
6
COULOMB
EXPLOSION
73
6.1
FRAGMENTATION
OF
NA
Q
CLUSTER
.
74
6.1.1
ENERGY
PARTITIONING
.
78
6.2
INCREASING
THE
CHARGE
OF
NAF
0
+
CLUSTER
.
78
7
PHASE
TRANSITION
IN
NUCLEAR
EVAPORATION
83
7.1
INTRODUCTION
.
83
7.2
EXPERIMENTAL
RESULTS
.
84
7.3
SIMULATION
WITH
MMMC
.
86
7.4
CONCLUSIONS
AND
DISCUSSION
.
89
8
SUMMARY
AND
CONCLUSIONS
91
8.1
MICROCANONICAL
TREATMENT
.
91
8.2
PHASE
TRANSITIONS
IN
CLUSTER
FRAGMENTATION
.
92
8.3
EXPERIMENTAL
ACCESSIBILITY
OF
THEORETICAL
PREDICTIONS
.
93
A
MONTE
CARLO
METHODS
95
B
MICROCANONICAL
WEIGHTS
IN
THE
MMMC
MODEL
97
CONTENTS
9
C
POLARIZATION
EFFECTS
IN
MANY-BODY
SYSTEMS
99
C.L
METHOD
OF
IMAGE
CHARGES
.
99
C.L.L
POINT
CHARGE
IN
PRESENCE
OF
CHARGED
CONDUCTING
SPHERE
.
100
C.L.
2
TWO
CHARGED
CONDUCTING
SPHERES
.
101
C.2
EXACT
SOLUTION
OF
COULOMB
INTERACTION
ENERGY
OF
SEVERAL
CONDUCTING
SPHERES
.
104
C.2.1
METHOD
.
104
C.2.2
THE
CHAIN
OF
CHARGES
.
106
C.2.3
ENERGY
CONVERGENCE
.
ILL
D
APPROXIMATION
BY
TWO-BODY
INTERACTIONS
117
E
POLARIZATION
EFFECTS
FOR
DIMERS
AND
TRIMERS
121
F
THE
MINIMAL
SURFACE
DISTANCES
DB
BETWEEN
THE
CLUSTERS
125
G
A
DIM
MODEL
FOR
SODIUM
CLUSTER
IONS
127
G.L
THE
CONCEPT
OF
DIM
.
127
G.2
SELF-CONSISTENT
CHARGE
DIM
MODEL
.
128
INDEX
143
ACKNOWLEDGEMENTS
145
LIST
OF
PUBLICATIONS
147
CURRICULUM
VITAE
149 |
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| discipline | Chemie / Pharmazie |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV011446635 |
| illustrated | Illustrated |
| indexdate | 2024-08-19T00:25:55Z |
| institution | BVB |
| isbn | 3896854275 |
| language | German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-007699659 |
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| open_access_boolean | |
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| physical | 148 S. Ill., graph. Darst. |
| publishDate | 1997 |
| publishDateSearch | 1997 |
| publishDateSort | 1997 |
| publisher | Wiss.-und-Technik-Verl. |
| record_format | marc |
| spelling | Schapiro, Olga Verfasser aut Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters Olga Schapiro 1. Aufl. Berlin Wiss.-und-Technik-Verl. 1997 148 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Zugl.: Berlin, Freie Univ., Diss., 1997 Phasenumwandlung (DE-588)4132140-6 gnd rswk-swf Metallcluster (DE-588)4128942-0 gnd rswk-swf Natrium (DE-588)4171239-0 gnd rswk-swf Mikrokanonische Gesamtheit (DE-588)4444250-6 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Natrium (DE-588)4171239-0 s Metallcluster (DE-588)4128942-0 s Mikrokanonische Gesamtheit (DE-588)4444250-6 s Phasenumwandlung (DE-588)4132140-6 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007699659&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Schapiro, Olga Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters Phasenumwandlung (DE-588)4132140-6 gnd Metallcluster (DE-588)4128942-0 gnd Natrium (DE-588)4171239-0 gnd Mikrokanonische Gesamtheit (DE-588)4444250-6 gnd |
| subject_GND | (DE-588)4132140-6 (DE-588)4128942-0 (DE-588)4171239-0 (DE-588)4444250-6 (DE-588)4113937-9 |
| title | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters |
| title_auth | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters |
| title_exact_search | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters |
| title_full | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters Olga Schapiro |
| title_fullStr | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters Olga Schapiro |
| title_full_unstemmed | Microcanonical phase transitions fragmentation and Coulomb explosion of metal clusters Olga Schapiro |
| title_short | Microcanonical phase transitions |
| title_sort | microcanonical phase transitions fragmentation and coulomb explosion of metal clusters |
| title_sub | fragmentation and Coulomb explosion of metal clusters |
| topic | Phasenumwandlung (DE-588)4132140-6 gnd Metallcluster (DE-588)4128942-0 gnd Natrium (DE-588)4171239-0 gnd Mikrokanonische Gesamtheit (DE-588)4444250-6 gnd |
| topic_facet | Phasenumwandlung Metallcluster Natrium Mikrokanonische Gesamtheit Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007699659&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT schapiroolga microcanonicalphasetransitionsfragmentationandcoulombexplosionofmetalclusters |