Catalyst deactivation 1991: proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991
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| Format: | Book |
|---|---|
| Language: | English |
| Published: |
Amsterdam [u.a.]
Elsevier
1991
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| Series: | Studies in surface science and catalysis
68 |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIII, 826 S. Ill., graph. Darst. |
| ISBN: | 0444888322 |
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| 245 | 1 | 0 | |a Catalyst deactivation 1991 |b proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 |c ed.: Calvin H. Bartholomew ... |
| 264 | 1 | |a Amsterdam [u.a.] |b Elsevier |c 1991 | |
| 300 | |a XIII, 826 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 1 | |a Studies in surface science and catalysis |v 68 | |
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| 650 | 4 | |a Catalyst poisoning |v Congresses | |
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| 830 | 0 | |a Studies in surface science and catalysis |v 68 |w (DE-604)BV000863094 |9 68 | |
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| _version_ | 1804123542787194880 |
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| adam_text | CONTENTS
Preface XIII
Review
Articles
(Plenary
Lectures)
In Situ Electron
Microscopy Studies of Catalyst Deactivation
R. T. K. Baker, Auburn University, USA
1
Thermal Stability of Catalyst Supports
D. L.
Trimm,
University of New South Wales, Australia
2 9
The Modeling of Catalyst Deactivation by Coke Formation
G. F. Froment,
University of Gent, Belgium
5 3
Promotion by Poisoning
J. R. Rostrup-Nielsen, Haldor Topsoe, Denmark
8 5
Topical Articles (Oral and Poster Presentations)
Carbon Deposition and Coking
Deactivation and Regeneration of Pt-Re/A^Oa Catalysts
J.
M. Parera
103
Effect of Steam on the Coking and on the Regeneration of Metal Catalysts:
A Comparative Study of Alumina-Supported Platinum, Rhenium,
Iridium
and
Rhodium Catalysts
D. Duprez. M. Hadj-Aissa and J.
Barbier
1 1 1
Deactivation of the Metal and Acid Functions of Pt/A^C^-CI Reforming
Catalysts by Coke Formation
J.
N.
Beltramini, T. J.
Wessel,
and R. Datta
1 1 9
Infrared Study of Carbon Deposition on Platinum-Tin/Alumina
J. Datka and R. P. Eischens
127
Coke and Product Profiles Along the Catalyst Bed in Reforming Reactions
S. C
Fung, C. A. Querini and
C. J.
McCoy
1 3 5
Relation Between Surface Structure and the Nature of Carbon Deposition
on Pt AI2O3 and
Р!-Ѕпа[2О3
Catalysts
Zhang Tao.
Zang
Jingling and Lin Liwu
1 4 3
Coking Kinetics of Reforming
R. L.
Mieviite
1 5 1
The Effect of Carbonaceous Depositions on Activity and Selectivity in
Hydrogénation
of an Unsaturated Aldehyde
B. Andersson.
M.
Eek
and A. Wrammerfors
1 6 1
The Effect of Hydrogen
Sulfide
on the Catalytic Action of Cobalt in Carbon
Gasification and Deposition Reactions
C. С.
Choti.
Ν. Μ.
Rodriguez and
R.
Т. К.
Baker
1 6 9
Hydrocarbon Steam Reforming Catalysts
-
Alkali Induced Resistance to
Carbon Formation
R. A.
Hadden.
J. C. Howe and
K. C. Waugh
1 7 7
VI
The Role of Sulfur in the Deposition of Carbon on Ruthenium and Nickel
Steam Reforming Catalysts
M. Masuda, T. Tabata, O. Okada, B. J. Wood, G. T.
Tong
and J. G. McCarty
1 85
Effects of Potassium on the Catalytic Behavior of Coked Nickel Catalysts in
Hydrogénation
and Hydrogenolysls Reactions
D. Duprez, M.
С
Demicheli,
J.
Barbier, P. Marecot, O. A.
Ferretti
and E.
N.
Ponzi
1 9 5
Reduced
Foulant Formation
During the Selective
Hydrogénation
of
C2,
СЗ
and C4 Acetylenes
J. T. Wehrll, D. J. Thomas, M. S. Wainwright, D. L.
Trimm
andN.
W. Cant
203
Kinetics and Deactivation of Unpromoted and Potassium-Promoted
Iron Fischer-Tropsch Catalysts at Low Pressure
(1
Atm)
S. A. Ellason and
C. H.
Bartholomew
2 1 1
Carbon Deposition Effects on CO
Hydrogénation
over Alumina-
and
Y
Zeolite-supported Cobalt Catalysts
S.-K.
Ihm,
D.-K.
Lee
219
The Constant-Parameter Arrhenius Plot In Coking and Poisoning
A. Bellare.
A. Raje,
and
D. B.
Dadyburjor
227
The Role of Deactivation in Decreasing the Surface Heterogeneity
of Pt SiO2 in the Isothermal
Hydrogénation
of Gaseous Cyclohexene
M. S. W.
Vong and P. Sermon
235
Coking-resistant Nickel Catalysts for Hydrocarbon Steam Reforming
Song Ruojun, Zhang Liangqu and Guo Shendu
2 4 3
The Deactivation of Tar Cracking Stones and of Commercial Methane Steam
Reforming Catalysts in the Upgrading of the Exit Gas from Steam
Fluidized
Bed Gasifiers of Biomass and Organic Wastes
J. Corelia. M. P.
Aznar,
J.
Delgado,
M.
P. Martinez, J. L.
Aragües
24 9
Resistance to Coking of Nickel-Alumina Catalysts
I. Chen and F. Chen
253
Hydrotreating Catalysts
Initial Coking and Deactivation of Hydrotreating Catalysts by
Rea!
Feeds
P. Wiwel. P. Zeuthen and A. C. Jacobsen
2 5 7
Implications of Analyses of Used Resid Demetallation Catalyst
H.D.Simpson
2 65
Hydrodemetallization in Resid Hydroprocessing
J. Barthoidy and P.
N.
Hannerup
273
Demetallization of Asphaltenes: Modelling Feed and Product
Molecular Size Distributions and Metal Distribution Parameters
E. L. Sughrue, R.
Adarme,
M. M.
Johnson,
C. J. Lord and M. D. Phillips
28 1
Topology of Coke Deposits in Spent Heavy Oil Processing Catalysts.
A Quantitative
Х
-Ray Photoeleciron Spectroscopy Study
K. P.
de
Jong, H. P.
С
E. Kuipers
and
J. A. R.
van Veen
2 8 9
Comparison of Hydrotreating Catalyst Deactivation by Coking
wim Vacuum Gas Oil vs. Anthracene
B. Muegge and
F. E.
Massoth
2 9 7
VII
Chemical
Stability of Hydrothermally Dealuminated
Y-Type
Zeolites:
A
Catalyst Manufacturer and User s Perspective
R.D.Bezman
305
The Effect of Diffusion on the Deactivation of Catalysts Used
for Hydrocracking Athabasca Bitumen
M. A. Altajam, J. F. Kriz and M.
Teman
3 1 5
Effect of Pore Diffusion on Deactivation in Resid Hydrodesulfurization
Y.-W. Chen, M.-C. Tsai and Y.-C. Kuo
3 23
Deactivation by Coke in Residuum Catalytic Cracking
ShaYingXun
327
Modeling and Kinetic Studies
Modelling of Hydrodemetallation
J.Wei
333
Combined Effects of Catalyst Deactivation and Intraparticle
Diffusion on the Dynamics of a Fixed Reactor
343
J. J. Yu and J. B. Butt
Thermal Deactivation of
Methanol
Synthesis Catalysts in a Slurry Reactor
G. W. Roberts, D. M. Brown, T. H. Hsiung and J. J. Lewnard
3 51
Deactivation of Cracking Catalysts with Vacuum Gas Oils
M. Forissier and J. R. Bernard
35 9
Dynamic Behavior of Catalytic Reactors with Activity Changes
M. Barto and
I. Hyánek
3 67
On the Kinetic Equation of Deactivation of Commercial Cracking (FCC) Catalysts with
Commercial Feedstocks
J. Corella and E. Frances
375
Modeling Deactivation of Large-pore Catalysts
J. M.
Loureiro
and A. E.
Rodrigues
383
Simultaneous Activation and Deactivation Phenomena in Isopropyl
Alcohol Dehydrogenation on a Cu/SiOj Catalyst
E. Agorreta, M. Salvador, J.
Santamaría
and
A. Monzón
3 9 1
Modeling of Simultaneous Deactivation Processes: Thioresistance
and Coking on Pt Based Catalysts
C. R.
Apesteguìa,
T. F. Garetto and A.
Borgna
3 9 9
Computer Simulated Deactivation of a Zeolite with Randomly
D.stnöuíed
Catalytic Sites
P. H. Nelson and D. M. Bibby
4 0 7
Mechanism and Analysis of Deactivation Data in Heterogeneous Polymerizations
M. Oiazar, J. M. Arandes, A. T.
Aguayo
and J. Bilbao
4 1 3
Oxides
Regeneration of Resd Hydrotreating Catalysts
F. T.Clark. A. L. Hensley. J.Z. Shyu, J.
A. Kaduk,
G.
J.
Ray 41 7
VIII
The Protecting Role of Antimony Oxide Against Deactivation of Iron
Molybdate in Oxidation Catalysts
Y. L. Xiong, R. Castillo, Ch. Papadopoulou, L.
Daza,
J.
Ladrière, P.
Ruiz
and B. Delmon
4 25
Heterogeneous Mo(VI) Catalysts for Liquid-Phase Epoxidation:
Evaluation of the Deactivation Patterns
E. Tempesti,
L. Giuffré,
F.
DiRenzo,
С.
Mazzocchia and P.
Gronchi
433
Deactivation of Heteropolyacid Catalysts
O. Watzenberger, Th. Haeberie, D. T. Lynch, and G. Emig
4 4 1
In-situ Control of Vanadyl
Pyrophosphate
Deactivation by Addition
of SO2 During C4-C5 Alkane Oxidation
G.
Centi,
J.
Gleaves,
G.
Golinelli,
S.
Perathoner and F. Trifiro
449
Study of the Deactivation of Supported Oxide Catalysts for Fuel Combustion
Using A Complex of Physical-Chemical Methods
D. A. Arendarskii, Z. R. Ismagilov, G. B. Barannik, V. A. Rogov
and E. A. Paukshtis
457
Deactivation of a Vanadium Oxide Catalyst for the Oxidation of Sulphur Dioxide
D. G. Klissurski,
I. G. Mitov, L. E.
Makedonski
and V. Bluskov
461
The Effect of Chromium on Deactivation of Alumina Supported Copper Catalysts
J.
Laine, F.
Severino, A. Lopez-Agudo and J.
L, G.
Fierro
467
Deactivation of Chromia-Alumina Catalyst for VOC Oxidation
S.K. Agarwal, J.J. Spivey, G. B. Howe, J.B. Butt, and
E. Marchand
4 75
Quantitative Description of Deactivation of AI2O3 for
N2O Decomposition by Addition of Na+,
LÌ+
and
F
P. Pomonis, S. Skaribas, A. Lykourghiotis and C. Kordoulis
479
Deactivation of
Claus
Catalysts
M.
Ziółek
485
Influence of Alkali Metals (Li and K) Addition to Ni/MgO Catalyst
A. Parmaliana, F. Arena, F.
Frusteri.
N.
Mondello and
N.
Giordano
48 9
Investigation of Deactivation of Industrial
Claus
Catalysts
F. B.
Kasumov
49 3
Poisoning
Mechanisms of Catalyst Poisoning by Sulfur Species
H. Wise
49 7
Hydrogénation
of 3-Methyl, Butenal on PtflOO): Reaction and
Deactivation Mechanism
50 5
С
M.
Pradier.
Y.
Berthier,
G.
Cordier and J. Oudar
Deactivation of Iron Oxide Catalysts for the Selective Oxidation
of Hydrogen
Sulfide
to Elemental Sulfur
P. j. van den Brink. A.
Scholten,
A. J. van
Dillen,
J. W.
Geus
E. Boellaard
and A.M. van
der Kraan
Poisoning of De-NO* SCR Catalyst by Flue Gases
trom
a Waste Incineration Plant
M.
Tokarz.
S.
Jarás
and
B. Persson
IX
Sulfur Poisoning of Mo-Promoted
Ni
Catalysts
G. J.
Siri,
G. S.
Marchettl,
О.
A. Ferretti
and M. G. Gonzalez
53 1
Sulfur Poisoning and Tolerance of
Methanol
Synthesis Catalysts
Chai Guoyong, Ai Dagang,
and Li Chengyue
53 9
The Effect of Adsorbed Sulfur on Heterogeneous Hydroformylatlon
over Rh,
Ni,
and RuCatalysts
M. W. Balakos,
S. I. Pien
and
S. S. C. Chuang
54 9
Comparative Study of the Deactivation of Group
VIII
Metal Catalysts
by Thiophene Poisoning in Ethylbenzene
Hydrogénation
A. Arcoya, A. Cortes, J. L. G.
Fierro
and X. L. Seoane
55 7
Sulfur Poisoning of Narrow Active Region Platinum/Alumina Catalyst Pellets
B. Remiarová, A. Brunovská
and M. Morbidelli
56 5
Sulfur Tolerance of
Mordente
Type Zeolite Containing Cupric Ions
for NO Reduction by NH3
I.-S. Nam, S.-W. Ham, H. Choi, and
Y. G.
Kim
5 7 3
The Mechanism of Sulfur-Poisoning of Pd(Pt)/AI2C>3 Catalysts
and Their Regeneration
An Li-Dun, Deng You-Quan, Xiao Tian-Cun, Xu Hong-Bing,
and Li Sheng-Li
57 7
Thioresistance of Reforming Catalysts In the Presence of Coking
L.
Gregoři.
A. Desmay, E. Agorreta, M. Menendez and
A. Monzón
5 8 1
Sintering
New Mechanisms of Sintering and
Redispersion
Induced by Spreading and Wetting
E.
Ruckenstein 58 5
Particle Shape Evolution in Gas Environments: Particle Shape Control
in Supported Metal Catalysis
W. H.
Lee, V. Petrova,
K. R.
Van Loon,
J. B.
Woodhouse,
C. M. Loxton, N. L. Finegan and R. I. Masel
59 7
Sintering of a Ni-Based Catalyst during CO
Hydrogénation:
Kinetics and Modeling
M. Agnelli. M.
Kolb,
С.
Nicot
and
С.
Mirodatos
60 5
Morphology Changes of Supported Rh Particles During
Thermal Treatments as Probed by Catalytic Measurements
W. E. Alvarez, R. J. Fenoglio, G. M. Nunez, A. J.
Rouco
and
D. E.
Resasco
61 3
Thermal Deactivation of the
PV fíhľJ-A 2O3 CeO2
Catalyst System
i. Onal
62 1
Non-Uniform Sintering in Oxyregeneration of Fixed Bed Catalytic Reactors
V.
Blasco,
С.
Royo,
M. Menendez, J.
Santamaría
and J. L. G.
Fierro
62
S
Towards a Better Understanding of Sintering Phenomena
¡n
Catalysis
G.
A. Fuentes and
E. D.
Gamas
6 3 7
Accelerated Sintering of
Pt
Catalysts in Reaction Atmosphere
for Rapid Estimation of Catalyst Life
Y. Murakami. S. Komai and T. Hattori
64 5
Effects of WO3 and La2O3 Addition on the Sintering and Phosphorous
Poisoning of
Pàly-/ 2O3
Catalysts for Automotive Emission Control
S. Y.
Lim,
T.
H.Jung,
К.
S.
Park,
J.
Y.
Sung
and S. J. Choung
65 3
Techniques
How Far Can Magnetic Methods Help in the Understanding
of Metal Catalyst Deactivation?
G. A. Martin
65 9
Cyclopropane Hydrogenolysis on Supported Pd Catalysts:
The Role of the Hydride and Variables that Affect Its Formation
H. E.
Rodriguez Cardenas and
D. E.
Damiani
66 7
ESCA
Study of Highly Dispersed Pd(Pt)/Al2C>3 Catalysts with Low Metal Loading
Deng You-Quan and An Li-Dun
6 75
Studies on the Degradation of Bimetallic
Pt-Sn/A^O^
Catalysts
in Regeneration Cycles
Fan Yining, Xu Zhusheng,
Zang
Jingling and Lin Liwu
68 3
Potassium Effects on the Deactivation by Carbon of Ruthenium Catalysts
T.
E. Hoost
and J. G. Goodwin, Jr.
691
The Conversion of
Ethylene
to Coke on Supported Platinum Catalysts
Investigated by 13C NMR
69 9
M.
Pruski,
X. Wu, M. W.
Smale,
В. С.
Gerstein and
T. S.
King
Monitoring the Performance of Ni-Mo-Alumina Catalyst in Lube
Hydrofinishing Through Catalyst Characterization
A. V. Ramaswamy and L. D. Sharma
70 7
Characterization of Metal Contaminants on Fluid Cracking Catalysts (FCC)
S. L. Sulb, E. V. R. Borgstedt, H.
Cao
and
M. L
Uccelli
7 1 7
Deactivation of Complete-Oxidation-Catalysts in Industrial Offgas:
Treatment and Its Prevention
T.Schmidt
723
Zeolites
Effects of Acidity and Metal Ensemble Size on Coke Formation
in PtNaY and PtCu/NaY by Methylcyclopentane Conversion
Z. Zhang. G.
Moretti,
G.
N.
Alameddin, and
W.
M. H.
Sachtier 72 7
Coking. Aging and Regeneration of Zeolites.
XII-
Composition of Coke
Formed on USHY during Phenol Alkylation with Methanol-Mode of Formation
M. Guisnet, I. Neves. F. R.
Ribeiro,
С.
Canaff, P. Magnoux and G. Perot
73 5
The Effect of Acidity on the Formaiion of Retained Residue from
1
-Hexene
over
USY
Zeolite Catalysts
J. R. Anderson. Y.-F. Chang and R. J. Western
74 5
Deactivation and the Role of
Extraframework
Aluminum in the Reactions
of 2-Methylpentane on Ultra-Stabilized
H Y
Zeolite
G. R.
Bamwenda,
W. A.
Groten, and
B. W.
Wojciechowski
75 3
Dc-activation Phenomena on Ti-Silicalite
G.
Petřini,
A. Cesana, G. De
Alberti.
F. Genoni, G.
Leofanti,
M.
Padovan,
G. Paparatto and P. Roffia
7 6 1
XI
Activation and Deactivation of Ga/HZSM-5 Catalysts in Propane
Aromatization at
773
К
P. Meriaudeau and
С
Naccache
7 6 7
The Deactivation of ZSM-5 in Catalytic Dewaxing
N.
Y. Chen, T. F. Degnan, J. D. Lutner and B. P. Pelrine
773
Deactivation of HZSM-5 Zeolite during
Methanol
Conversion:
Kinetic Probing of Pore-Architecture and Acidic Properties
7 83
H.
Schulz,
D.
Barth
and
Z.
Siwei
Selective Poisoning of ZSM-5 by Nitrogen Heterocycles
L. D.
Rollmann 791
Deactivation of Sulfur Tolerant
Water-Gas
Shift Catalysts
Based on Ni-Mo-Y Zeolites
M. Laniecki and W. Zmierczak
79 9
FCC Catalyst Demetallization
F. J.
Elvin
803
Effect of the
Hydrothermal
Treatment of
Y
Zeolites on Coke Formation
F.
Machado,
P. Magnoux and M. Guisnet
8 0 7
Cracking Activity Measurements of Zeolite Catalysts with Catalytic Deactivation
J. Medina and I. Schifter
8 1 1
Deactivation of Zeolite Catalysts In
Methanol
Conversion to Hydrocarbons
Zhongmin Liu, Guoquan Chen, Juan Liang, Quingxia Wang and Guangyu
Cal
8 1 5
Author Index
8 1 9
Studies in Surface Science and Catalysis (Other Volumes in the Series)
823
|
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| building | Verbundindex |
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| genre | (DE-588)1071861417 Konferenzschrift 1991 Evanston Ill. gnd-content |
| genre_facet | Konferenzschrift 1991 Evanston Ill. |
| id | DE-604.BV009127158 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T17:31:26Z |
| institution | BVB |
| isbn | 0444888322 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-006049669 |
| oclc_num | 23584633 |
| open_access_boolean | |
| owner | DE-91 DE-BY-TUM DE-703 |
| owner_facet | DE-91 DE-BY-TUM DE-703 |
| physical | XIII, 826 S. Ill., graph. Darst. |
| publishDate | 1991 |
| publishDateSearch | 1991 |
| publishDateSort | 1991 |
| publisher | Elsevier |
| record_format | marc |
| series | Studies in surface science and catalysis |
| series2 | Studies in surface science and catalysis |
| spelling | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 ed.: Calvin H. Bartholomew ... Amsterdam [u.a.] Elsevier 1991 XIII, 826 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Studies in surface science and catalysis 68 Catalyseurs - Empoisonnement ram Catalyst poisoning Congresses Desaktivierung (DE-588)4260078-9 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf (DE-588)1071861417 Konferenzschrift 1991 Evanston Ill. gnd-content Katalysator (DE-588)4029919-3 s Desaktivierung (DE-588)4260078-9 s DE-604 Bartholomew, Calvin H. Sonstige oth Studies in surface science and catalysis 68 (DE-604)BV000863094 68 Digitalisierung TU Muenchen application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006049669&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 Studies in surface science and catalysis Catalyseurs - Empoisonnement ram Catalyst poisoning Congresses Desaktivierung (DE-588)4260078-9 gnd Katalysator (DE-588)4029919-3 gnd |
| subject_GND | (DE-588)4260078-9 (DE-588)4029919-3 (DE-588)1071861417 |
| title | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 |
| title_auth | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 |
| title_exact_search | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 |
| title_full | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 ed.: Calvin H. Bartholomew ... |
| title_fullStr | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 ed.: Calvin H. Bartholomew ... |
| title_full_unstemmed | Catalyst deactivation 1991 proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 ed.: Calvin H. Bartholomew ... |
| title_short | Catalyst deactivation 1991 |
| title_sort | catalyst deactivation 1991 proceedings of the 5th international symposium evanston il june 24 26 1991 |
| title_sub | proceedings of the 5th International Symposium, Evanston, IL, June 24 - 26, 1991 |
| topic | Catalyseurs - Empoisonnement ram Catalyst poisoning Congresses Desaktivierung (DE-588)4260078-9 gnd Katalysator (DE-588)4029919-3 gnd |
| topic_facet | Catalyseurs - Empoisonnement Catalyst poisoning Congresses Desaktivierung Katalysator Konferenzschrift 1991 Evanston Ill. |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006049669&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000863094 |
| work_keys_str_mv | AT bartholomewcalvinh catalystdeactivation1991proceedingsofthe5thinternationalsymposiumevanstoniljune24261991 |