Catalytic activation of dioxygen by metal complexes:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Dordrecht u.a.
Kluwer
1992
|
| Schriftenreihe: | Catalysis by metal complexes
13 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | VIII, 396 S. graph. Darst. |
| ISBN: | 079231896X |
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Datensatz im Suchindex
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| adam_text | IMAGE 1
TABLE OF CONTENTS
PREFACE IX
1. DIOXYGEN COMPLEXES 1
INTRODUCTION 1
1.1. THE O 2 MOLECULE 4
1.1.1. BONDING 4
1.1.2. THERMODYNAMIC DATA 5
1.1.3. REACTIVITY OF O 2 8
1.2. STRUCTURE AND BONDING IN DIOXYGEN COMPLEXES 10
1.3. SPECTROSCOPY OF DIOXYGEN COMPLEXES 24
1.3.1. ELECTRONIC SPECTRA 24
1.3.2. INFRARED AND RAMAN SPECTRA 27
1.3.3. - ESR SPECTROSCOPY 32
1.3.4. 17O-NMR SPECTROSCOPY 33
1.4. EQUILIBRIA OF DIOXYGEN COMPLEXES 37
1.5. KINETICS AND MECHANISMS OF DIOXYGEN COMPLEX FORMATION AND
DECOMPOSITION 48
1.5.1. FORMATION OF SUPEROXO COMPLEXES 49
1.5.2. FORMATION AND DECOMPOSITION OF U-PEROXO COMPLEXES 51
1.5.3. DECOMPOSITION OF U-PEROXO COMPLEXES OF COBALT 59
REFERENCES 61
2. CATALYTIC OXIDATION OF SATURATED HYDROCARBONS WITH O 2 74
INTRODUCTION 74
2.1. METAL-FREE SYSTEMS 74
2.1.1. INITIATED CHAIN REACTIONS 74
2.1.2. BASE-CATALYZED AUTOXIDATIONS 77
2.2. METAL COMPLEXES AS CATALYSTS 80
2.2.1. SYSTEMS INVOLVING DIRECT OXIDATION BY METAL IONS 80
2.2.2. METAL COMPLEX CATALYZED OXIDATIONS 83
2.2.3. METALLOPORPHYRIN CATALYZED OXIDATIONS 90
2.2.3.1. PHIO AS OXYGEN SOURCE 90
2.2.3.2. DIOXYGEN AS TERMINAL OXIDANT 92
2.2.4. GIF TYPE SYSTEMS 95
SUMMARY 102
REFERENCES 103
3. CATALYTIC OXIDATION OF ALKENES WITH O 2 109
INTRODUCTION 109
3.1. EPOXIDATIONS 110
3.1.1. STOICHIOMETRIC EPOXIDATIONS WITH PEROXOMETAL COMPLEXES 110
IMAGE 2
3.1.2. METALLOPORPHYRIN CATALYZED EPOXIDATIONS USING O-ATOM
TRANSFER REAGENTS 113
3.1.3. METALLOPORPHYRIN CATALYZED EPOXIDATION WITH DIOXYGEN 124 3.1.4.
REDUCTIVE O 2-ACTIVATION WITH METALLOPORPHYRINS 125
3.1.5. NON-PORPHYRIN CATALYSTS FOR EPOXIDATION 130
3.1.6. EPOXIDATION WITH NITRO COMPLEXES OF METALS 132
3.2. CATALYTIC OXIDATION OF OLEFINS TO KETONES AND ALDEHYDES 134
3.2.1. WACKER TYPE OXIDATION OF OLEFINS 134
3.2.2. CATALYTIC OXYGENATION OF OLEFINS TO KETONES 137
3.2.2.1. RHODIUM CATALYSTS 137
3.2.2.2. COBALT SCHIFF-BASE CATALYSTS 144
3.2.2.3. RUTHENIUM CATALYSTS 149
3.2.3. OLEFIN OXYGENATION WITH C=C BOND CLEAVAGE 149
3.2.4. OXYGENATION OF INDOLE DERIVATIVES (TRYPTOPHAN MODELS) 151 3.3.
ALLYLIC OXIDATION 160
3.4. FORMATION OF GLYCOLS AND CARBONATES 161
3.5. REDOX HYDRATION OR OXYGENATION UNDER REDUCTIVE CONDITIONS 162
3.6. EFFECT OF O 2 ON OLEFIN METATHESIS 165
3.7. CATALYTIC OXIDATION OF ALKYNES 166
SUMMARY 169
REFERENCES 171
4. CATALYTIC HYDROXYLATION OF AROMATIC HYDROCARBONS WITH O 2 181
INTRODUCTION 181
4.1. BENZENE HYDROXYLATION 181
4.2. MECHANISM OF BENZENE HYDROXYLATION 185
4.3. HYDROXYLATION OF M -XYLENE DERIVATIVES 188
SUMMARY 192
REFERENCES 193
5. CATALYTIC OXIDATION OF PHENOLS 196
5.1. BASE-CATALYZED OXIDATION OF SUBSTITUTED PHENOLS 196
5.2. METAL COMPLEXES AS CATALYSTS FOR OXIDATION OF ALKYL-SUBSTITUTED
PHENOLS 200 5.2.1. COBALT(II) SCHIFF-BASE COMPLEXES AS CATALYSTS 200
5.2.2. MECHANISM OF CATALYTIC OXIDATION OF HINDERED PHENOLS IN THE
PRESENCE OF VARIOUS METAL COMPLEXES 207
5.2.2.1. COBALT(II) SCHIFF-BASE COMPLEXES 207
5.2.2.2. BIS(BIPYRIDYL)COBALT(II) 218
5.2.2.3. COBALT(II) POLYAMINE CHELATES 220
5.2.2.4. PENTACYANOCOBALTATE(H) 223
5.2.2.5. COPPER CATALYSTS 224
5.2.2.6. METALLOPORPHYRINS 226
5.2.2.7. METALLOPHTHALOCYANINES 227
5.2.2.8. OTHER CATALYST SYSTEMS 228
5.3. CATALYTIC OXIDATIVE COUPLING OF PHENOLS 229
IMAGE 3
5.4. CATALYTIC HYDROXYLATION OF PHENOLS (TYROSINASE MODELS) 233
5.4.1. TYROSINASE 233
5.4.2. COPPER COMPLEXES 234
5.4.3. IRON COMPLEXES 236
5.4.4. COBALT COMPLEXES 239
5.4.5. PD AND RU COMPLEXES 241
SUMMARY 241
REFERENCES 243
6. CATALYTIC OXIDATION OF CATECHOLS 249
6.1. DISCOVERY AND TYPES OF OXYGENASES 249
6.2. CATALYTIC OXIDATIVE DEHYDROGENATION OF CATECHOLS TO O -QUINONES 252
6.3. CATALYTIC OXIDATIVE CLEAVAGE OF CATECHOLS 257
6.3.1. BASE CATALYZED OXIDATIONS 257
6.3.2. COPPER CATALYSTS 259
6.3.3. IRON CATALYSTS 271
6.3.3.1. DIOXYGENASE ENZYMES 271
6.3.3.2. NON-HEME IRON DIOXYGENASE MODELS 273
6.3.4. VANADIUM CATALYSTS 282
6.3.5. COBALT CATALYSTS 285
6.3.6. COMPLEXES OF OTHER METALS AS CATALYSTS 289
SUMMARY 291
REFERENCES 292
7. CATALYTIC OXIDATION OF ALCOHOLS WITH O 2 297
7.1. DEHYDROGENATION OF ALCOHOLS WITHOUT O 2 297
7.1.1. RHODIUM AND IRIDIUM COMPLEXES 297
7.2. OXIDATIVE DEHYDROGENATIONS WITH O 2 298
7.2.1. MOLYBDENUM AND VANADIUM COMPLEXES 298
7.2.2. RHODIUM COMPLEXES 298
7.2.3. RHODIUM-COPPER COMPLEXES 298
7.2.4. RUTHENIUM COMPLEXES 299
7.2.5. COPPER COMPLEXES 301
7.2.6. PALLADIUM COMPLEXES 304
7.2.7. MANGANESE COMPLEXES 304
7.2.8. COBALT COMPLEXES 304
SUMMARY 305
REFERENCES 306
8. CATALYTIC OXIDATION OF DIOLS AND POLYOLS WITH O 2 308
8.1. ASCORBIC ACID 308
8.2. DIOLS 312
8.3. POLYOLS AND SUGARS 315
SUMMARY 316
REFERENCES 317
IMAGE 4
9. CATALYTIC OXIDATION OF ALDEHYDES AND KETONES WITH O 2
9.1. ALDEHYDES
9.2. ACETALS
9.3. KETONES
9.4. ACYLOINS
SUMMARY REFERENCES
10. CATALYTIC OXIDATION OF NITROGEN COMPOUNDS WITH O 2 10.1.
DEHYDROGENATION OF NITROGEN-CONTAINING COMPOUNDS
10.1.1. AMINO ACIDS AND PEPTIDES 10.1.2. ALIPHATIC MONOAMINES 10.1.3.
DIAMINES AND POLYAMINES 10.1.4. MACROCYCLES 10.1.5. AROMATIC AMINES
10.1.5.1. AROMATIC MONOAMINES 10.1.5.2. AROMATIC DIAMINES 10.1.5.3. O
-SUBSTITUTED ANILINES 10.1.6. HYDRAZOBENZENE AND MISCELLANEOUS
(AROMATIC) NITROGEN
COMPOUNDS 344
10.2. OXYGEN INSERTIONS INTO NITROGEN-CONTAINING COMPOUNDS 346
10.2.1. ALKYLAMINES 346
10.2.2. ARYLAMINES (OXIDATIVE DEALKYLATION) 348
10.2.3. AMINO ACIDS (PYRIDOXAL CATALYSIS) 351
10.2.4. PEPTIDES 353
10.2.5. MISCELLANEOUS NITROGEN COMPOUNDS 355
SUMMARY 359
REFERENCES 360
11. OXIDATION AND CO-OXIDATION OF TERTIARY PHOSPHINES 363
SUMMARY 368
REFERENCES 369
12. OXIDATION OF SULFUR COMPOUNDS 371
12.1. CATALYTIC OXIDATION OF THIOETHERS 371
12.2. CATALYTIC OXIDATION OF THIOLS 374
SUMMARY 383
REFERENCES 384
ABBREVIATIONS 387
SUBJECT INDEX 393
|
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| id | DE-604.BV008162736 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T17:15:34Z |
| institution | BVB |
| isbn | 079231896X |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-005385432 |
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| physical | VIII, 396 S. graph. Darst. |
| publishDate | 1992 |
| publishDateSearch | 1992 |
| publishDateSort | 1992 |
| publisher | Kluwer |
| record_format | marc |
| series | Catalysis by metal complexes |
| series2 | Catalysis by metal complexes |
| spelling | Simándi, László I. Verfasser aut Catalytic activation of dioxygen by metal complexes by László I. Simándi Dordrecht u.a. Kluwer 1992 VIII, 396 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Catalysis by metal complexes 13 Catalysis Metal complexes Oxygen Aktivierung Chemie (DE-588)4141761-6 gnd rswk-swf Katalyse (DE-588)4029921-1 gnd rswk-swf Übergangsmetallkomplexe (DE-588)4131837-7 gnd rswk-swf Oxygenierung (DE-588)4319631-7 gnd rswk-swf Sauerstoffmolekül (DE-588)4386564-1 gnd rswk-swf Oxygenierung (DE-588)4319631-7 s Katalyse (DE-588)4029921-1 s Übergangsmetallkomplexe (DE-588)4131837-7 s DE-604 Sauerstoffmolekül (DE-588)4386564-1 s Aktivierung Chemie (DE-588)4141761-6 s Catalysis by metal complexes 13 (DE-604)BV001899776 13 OEBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=005385432&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Simándi, László I. Catalytic activation of dioxygen by metal complexes Catalysis by metal complexes Catalysis Metal complexes Oxygen Aktivierung Chemie (DE-588)4141761-6 gnd Katalyse (DE-588)4029921-1 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd Oxygenierung (DE-588)4319631-7 gnd Sauerstoffmolekül (DE-588)4386564-1 gnd |
| subject_GND | (DE-588)4141761-6 (DE-588)4029921-1 (DE-588)4131837-7 (DE-588)4319631-7 (DE-588)4386564-1 |
| title | Catalytic activation of dioxygen by metal complexes |
| title_auth | Catalytic activation of dioxygen by metal complexes |
| title_exact_search | Catalytic activation of dioxygen by metal complexes |
| title_full | Catalytic activation of dioxygen by metal complexes by László I. Simándi |
| title_fullStr | Catalytic activation of dioxygen by metal complexes by László I. Simándi |
| title_full_unstemmed | Catalytic activation of dioxygen by metal complexes by László I. Simándi |
| title_short | Catalytic activation of dioxygen by metal complexes |
| title_sort | catalytic activation of dioxygen by metal complexes |
| topic | Catalysis Metal complexes Oxygen Aktivierung Chemie (DE-588)4141761-6 gnd Katalyse (DE-588)4029921-1 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd Oxygenierung (DE-588)4319631-7 gnd Sauerstoffmolekül (DE-588)4386564-1 gnd |
| topic_facet | Catalysis Metal complexes Oxygen Aktivierung Chemie Katalyse Übergangsmetallkomplexe Oxygenierung Sauerstoffmolekül |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=005385432&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV001899776 |
| work_keys_str_mv | AT simandilaszloi catalyticactivationofdioxygenbymetalcomplexes |