Far-infrared spectroscopy:
Saved in:
| Main Authors: | , |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
New York
Wiley
1971
|
| Series: | Wiley series in pure and applied optics
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIX, 797 S. Ill., graph. Darst. |
| ISBN: | 0471613134 |
Staff View
MARC
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| 100 | 1 | |a Möller, Karl Dieter |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Far-infrared spectroscopy |c Karl Dieter Möller ; Walter G. Rothschild |
| 264 | 1 | |a New York |b Wiley |c 1971 | |
| 300 | |a XIX, 797 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 0 | |a Wiley series in pure and applied optics | |
| 650 | 7 | |a Infraroodspectrometrie |2 gtt | |
| 650 | 7 | |a Materia Condensada (Espectroscopia) |2 larpcal | |
| 650 | 7 | |a Otica, Holografia, Laser E Cor |2 larpcal | |
| 650 | 4 | |a Spectroscopie infrarouge | |
| 650 | 4 | |a Infrared Rays | |
| 650 | 4 | |a Infrared spectroscopy | |
| 650 | 4 | |a Spectrum Analysis | |
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| 689 | 0 | |5 DE-604 | |
| 700 | 1 | |a Rothschild, Walter G. |e Verfasser |4 aut | |
| 856 | 4 | 2 | |m Digitalisierung UB Regensburg |q application/pdf |u http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000570507&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |3 Inhaltsverzeichnis |
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Record in the Search Index
| _version_ | 1804115364549754880 |
|---|---|
| adam_text | Contents
1
Grating Spectrometers
A. Introduction
1
B.
Optical Layout of Spectrometers
2
a. General
2
b. Littrow Mount
2
с
Czerny-Turner Mount
4
d. Ebert-Fastie Mount
6
e. f-Number
of the Monochromator
8
С
Gratings
8
a. General
8
b. Grating Formula and Intensity Distribution
9
с
Spectral Slit Width
15
D. Energy Limitations on the Resolving Power
16
E. Filters
19
a. Introduction
19
b. Attenuation Requirements
20
с
Elimination of Short-Wavelength Radiation
22
d. Reflection Crystal Filters
{Reststrahlen
Filters)
24
e. Transmission Crystal-Powder Filters
24
ƒ.
Reflection Filter Gratings
30
g. Transmission Filter Gratings
31
h. Metal Mesh Reflection Filters
35
j. Interference Filters
41
F. Checks for False Radiation
41
ix
x
Contents
G.
Polarization of Spectrometer Components
42
a. Reflection Filter Gratings
43
b. Diffraction Gratings
44
c. Crystal Reflection Plates
44
H. Wavelength Calibration
44
a. General
44
b. Calibration with Water Vapor
46
с
Calibration with Methyl Chloride and Other Compounds
49
References
52
2
Common Parts of Grating Spectrometers and Interferometers and
Some Accessories
A. Sources
55
B. Detectors
57
a. Detector Characterization
57
b. Golay Detector
58
с
Liquid-Helium Temperature Detectors
60
1.
Introduction and General Considerations
61
2.
Carbon Resistance and Doped Germanium Bolometers
61
3.
Indium-Antimonide Detector
64
4.
Doped Germanium Photoconducting Detectors
66
5.
Comparison of the Liquid-Helium Temperature Detec¬
tors and Problems of Their Use
67
С
Light-Pipes
68
D. Conical Light-Pipes (Channel Condensers)
72
E. Polarizers
75
a. Linear Polarizers
75
1.
Pile-of-Plates Polarizer
75
2.
Wire-Grating Polarizer
76
3.
Pyrolytic Graphite Transmission Polarizer
78
b. Circular and Elliptical Polarizers
79
1.
Soleil
Compensator
79
2.
Polarizer Using a Magnetic Field
81
F. Multiple-Path Cells
82
G. Image Transformer
86
H. Vacuum System and Cryogenic Equipment
87
References
88
Contents xi
3 Fabry-Perot
Interference Filters and Tunable Fabry-Perot
Etalon
A. Fabry-Perot Interference Filters and Spectrometer
90
a. General
90
b. Airy Formula and Finesse
90
B. Reflectors for the Far-Infrared
92
a. Metal Gratings in Empty Space
93
b. Grating and Mesh in the Vicinity of a Dielectric Medium
96
с
Metal Meshes and Their Equivalent Circuit Representation
97
d. Phase Measurements
107
e. Fabrication of Meshes
107
С
Interference Filters
109
a. Theory of Two-Mesh Filters
109
b. Formulas for the Calculation of the Transmittance of Multi-
Mesh Filters 111
с
Construction of Fabry-Perot Interference Filters
111
d. Measurements on Interference Filters and Comparison with
Theory
113
e. Phase Measurements with Interference Filters
122
D. Tunable Fabry-Perot Interferometer
123
E. Fabry-Perot Interferometer in Higher Orders
125
F. Comparison of a Grating and a Fabry-Perot Spectrometer
under Energy-Limited Conditions
125
References
127
4
Fourier Transform Spectroscopy
A. Introduction
128
B. Interferogram Function and Fourier Transformation
129
C. Finite Path Difference, Apodization, and Resolution
131
D. Sampling
136
E. Phase Error and Its Correction. Maladjustment
139
F. Advantages and Disadvantages of Fourier Transform
Spectroscopy Compared to Grating Spectroscopy
144
G. Finite Aperture, Sensitivity, and Dynamic Range of the
Recording System
145
H. Michelson Interferometer
146
Contents
I. Lamellar-Grating Interferometer
151
J.
Interferometry
in the Asymmetric Mode
156
a. Introduction
156
b. Theory and Experimental Results
157
References
160
5
Low-Frequency Stretching and Bending Fundamentals
A. Introduction
163
B. Disulfur Dichloride and Disulfur Dibromide
164
C. Carbon Suboxide and Carbon Subsulfide
167
D. 1,4-Dioxadiene
173
E. Molecules Containing Fluorine
174
a. Xenon Difluoride
174
b. Xenon Tetrafluoride
178
c. Phosphorous Pentafluoride and Arsenic Pentafluoride
179
F. Metal Carbonyls
183
G. Halogen Derivatives of
Alkyl
Compounds
186
References
195
6
Far-Infrared Spectra of Hydrogen-Bonded Systems
A. Introduction
198
B. Self-Associated Phenols
200
С
Hydrogen Bonds between Phenols and Amines
207
D. Hydrogen Bonding in Carboxylic Acids
211
E. Solvent Effects on Hydrogen-Bond Frequencies
214
F. Concluding Remarks
217
References
-217
7
Skeletal Modes of Strained-Ring Systems
A. Introduction
218
B. Theoretical Considerations
220
C. Symmetric Ring-Puckering Potential Functions
221
a. Cyclobutane
and Perfluorocyclobutane
221
b. Tr
¿methylene
Oxide
222
Contents xiii
c.
Cyclobutanone
227
d.
Perfluorocylobutanone
227
e. Trimethylene
Sulfide 228
f.
Dùcetene,
ß-Propiolactone, 1 ¿-Tetrafluoro-l,3-dithietane,
3-Methyleneoxetane 229
D. Potential
Function and Ring Conformation
230
E. Nonsymmetrical
Ring-Puckering
Potential
Functions
232
a. Introduction
232
b.
Bromocyclobutane
234
c. Chlorocyclobutane
237
d.
Deuterated Bromo-
and Chlorocyclobutanes
239
e. Fluorocyclobutane
239
f.
Conclusions
239
F. Pseudorotation
of Five-Membered Rings
240
a. Introduction
240
b. Cyclopentane
244
c. Tetrahydrofuran
245
d. 2,5-Dihydrofuran
250
References
253
8
Torsional Motions with Periodic Potential Barriers
A. Introduction
256
B. One-Top Molecules with Threefold Barriers
256
a. Introduction
256
b. Principal Axis Method
(РАМ)
and the Hamiltonian of the
Internal Rotation for a Symmetric-Top Molecule
257
c. Hamiltonian in the Internal Axis Method
(IAM)
for a
Symmetric-Top Molecule
260
d. Potential Energy
262
e. Asymmetric-Top Molecules without Structural Symmetry
and the Principal Axis Method
(РАМ)
262
ƒ.
Asymmetric-Top Molecules with a Plane of Symmetry and
the Internal Axis Method
(IAM)
263
g.
Far-Infrared Spectrum of Methyl Alcohol
264
h. Far-Infrared
Torsionai
Vibration Spectra of Various
Molecules
269
i. Selection Rules
273
j. Spectra and Calculations of the Potential Function
Constants
275
xjv
Contents
C.
Two-Top Molecules of C2v and Cs Symmetry with Threefold
Barriers
279
a. Kinetic and Potential Energy
279
b. Harmonic Oscillator Approximation
281
с
Periodic Potential Model. Symmetry Properties, Energy
Level Scheme, Selection Rules
283
d. Spectra and the Calculation of the Potential Function
Constants
285
D. Three-Top Molecules
(Сз,,)
With Threefold Barriers
288
a. Theoretical Considerations
288
b. Spectra and Potential Barriers
289
E. Twofold Barriers
291
a. Hydrogen Peroxide and Deuterated Hydrogen Peroxide
291
b. Twofold Barriers about a Carbon-Carbon Bond
298
с
Meta-
and
Ortho-Substituted Benzaldehyde
and Furan-2-
aldehyde
300
References
301
9
Pure Rotational Spectra of Vapors: Water
A. Introduction
303
B. Observed Spectra of Atmospheric Water Vapor
304
a. Spectral Region
300
to
150
cm x
304
b. Spectral Region
150
to
100
cm~ 1
304
с
Spectral Region 111 to
72
cm~
* 308
d. Spectral Region
80
to
60
cm~l
308
e. Spectral Region
64
to
50
cm 1
309
ƒ.
Spectral Region
53
to
32
cm 1
309
g. Spectral Region
30
to
10
cm
л
310
C.
Computation and Tabulation of Pure Rotational Transitions
of Water Vapor
313
D. Tabulation of Pure Rotational Water Vapor Transitions
between
12
and
305
cm~
λ
317
References
324
10
Collision-Induced Spectra at Long Wavelengths
A. Introduction
325
Contents
В.
Theory of Induced Absorption
330
a. Absorption Coefficients, Cluster Functions, and Induced
Vibrational-Rotational Transitions
330
b. Induced Pure Rotational Transitions
342
с
Induced Pure Translational and Translational-Rotational
Absorption
343
С
Experimental Observations
348
a. Pure Translational Absorption. Helium-Argon and Neon-
Argon Mixtures
348
b. Rotational-Translational Absorption
358
1.
Hydrogen
358
2.
Nitrogen, Oxygen
359
с
Pressure-Induced Quadrupole Spectra. Hydrogen Chloride
and Hydrogen Bromide
362
d. Induced Rotation- Translation Spectra in Liquids. Solutions
of
H
2,
D2, and
HD in
Liquid
Ar 367
References
371
11
Rotational-Translational Motion in Condensed Phases
A. Introduction
373
B. The
Heisenberg
Picture
375
C. Rotational Motion from the Band Shapes of Vibrational
Transitions
380
a. Introduction
380
b. Rotational Motion of
Methylene
Chloride (CH2Cl2) in
Polystyrene
382
с
Rotational Motion in Liquid Methyl Iodide
386
D. Rotational Motion from the Band Shapes of Rotational
Spectra
389
a. Introduction
389
b. Individual Molecules. The Hydrogen Halides, Water, and
Ammonia
394
с
Rotational Motion of a Distortion in Liquid Carbon
Tetrachloride 399
d.
Molecular Complexes and Clusters in Liquid Phases
403
References
411
12
Far-Infrared Spectra of Diatomic Cubic Crystals
A. Introduction
412
,vj Contents
B.
Classical Description of Crystal Spectra
413
a. Dielectric Constant, Refractive Index, and Extinction
Coefficient
413
b. Dispersion Formulas
416
c. Kramers-Kronig Relations
419
d. Dispersion Measurements on Alkali Halides
420
C. Effects of Periodicity
440
a. Lattice Modes of Cubic Crystals
440
b. Effects of Sample Geometry
447
с
Selection Rules and General Appearance of the Spectra
451
D. Temperature Dependence of Phonon Interactions
460
a. Occupation Number
460
b. Frequency and Temperature Dependence of the Damping
Constant
461
E. Structure Faults and Phonon Processes
465
a. Supertransparency
465
b. Diatomic Linear Chain with Symmetrically Placed Lattice
Faults
465
References
470
13
Far-Infrared Spectra op Polyatomic Crystals
A. Introduction
472
B. Lattice Vibration Spectra of NiF2, CoF2, and FeF2
475
a. Factor Group Analysis. General Principles
475
b. Derivation of the Symmetry Species of the Fundamentals
480
с
Experimental Results
490
С
Lattice Vibrations of KNiF3
492
D. Lattice Vibration in Crystalline Polyethylene
494
E. Spectra of Crystalline Nitrogen and Carbon Monoxide
497
F. Crystal Spectra of Complexes
500
a. Silver
Ealide
Complexes of the Types RAg2X3, RAgX2,
and RtAgXz
500
b. Metal-Ligand Force Constants of Acetylacetonates
505
G. Temperature and Pressure Dependence of Lattice Modes
511
H. Vibrational Spectra of Orientationally Disordered Crystals.
Translational Lattice Vibrations of Ice Ic and
Ih
516
References
522
Contents xvii
Appendix I Impurity-Induced Lattice Absorption in the Far-Infrared,
by A. J. Sievers
A. Introduction
525
B. Impurity-Induced Absorption
531
С
Local Modes
534
D. Gap Modes
539
a. Monatomic Impurities
539
b. Molecular Impurities
544
E. Resonant Modes
544
a. Model
544
b. Observations
548
с
Stress Effects
551
d. Temperature Effects
553
F. Summary
554
References
554
Appendix II Dielectric Properties and Optical Phonons in Para- and
Ferro-electric Perovskites, by
C. H.
Perry
A. Introduction
557
B. Lattice Modes Based on the Shell Model
560
C. Crystal Symmetry and Species of the Vibrational Modes
567
D. Infrared Reflection Measurements
568
E. Analysis of Reflection Spectra by Means of a Kramers-
Kronig Relation or a Fit with a Classical Dispersion
Formula
574
a. Kramers-Kronig Analysis
574
b. Classical Dispersion Analysis
577
F. The Dielectric Response Function
582
G. Paraelectric Crystals
586
H. Ferroelectric Crystals
586
I. Conclusions
589
References
590
Appendix III Magnetic Phenomena in the Far-Infrared, by Isaac F.
Silvera
A. Introduction
592
xviii Contents
B.
Cryostates
594
C.
Antiferromagnetic
Insulators
595
D.
Spin Wave Excitation Spectra
597
E. Single-Magnon
Absorption
600
F. Two-Magnon Absorption
603
G. Crystalline Electric Field Effects
605
References
610
Appendix IV Far-Infrared Spectroscopic Studies of Semiconductors,
by R. Kaplan
A. Optical Lattice Vibrations and Free Carrier Effects
612
a. Transmission and Reflection Measurements
612
b. Measurement of Emission
616
B. Impurity Absorption and Photoconductivity
619
a. Energy States of Impurity Atoms in Germanium and Silicon
620
b. Hydrogenic Impurity States in Indium Antimonide
625
с
Far-Infrared Resonant Absorption due to Donor Impurity
Pairs in Silicon
630
С
Cyclotron Resonance Investigations
630
a. Cyclotron Resonance Studies Using Mixed Microwave-
Optical Techniques
631
b. Cyclotron Resonance Studies Using Purely Optical
Techniques
635
D. Coupled Phonon—Free Carrier Modes
640
a. Polaron Modes
641
b. Coupled Collective Plasma Cyclotron—Longitudinal Optical
Phonon Modes
643
References
645
Appendix V Superconductivity, by Gerhart K.
Gaulé
A. Introduction
647
a. Far-Infrared Radiation and Superconductivity as Low-
Energy Phenomena
647
b. General Features of Low-Temperature Optical and
Electronic Systems. Noise
647
с
Cooling Requirements for Superconductors
650
Contents xix
B.
Homogeneous Superconductors in Weak Fields
652
a. The Two-Fluid Model. Resistive Bolometers
653
b. The Energy Gap and Its Optical Significance
656
C. Homogeneous Superconductors in Strong Fields
665
D. Composite and Weakly Coupled Superconductors
666
E. Superconductivity in Conjunction with Other Solid State
Effects. Parametric Thermometer
669
References
670
Appendix VI Rapid-Scan Fourier Spectroscopy, by Ernest V.
Loewenstein
A. Introduction
672
B. Order-Sorting and Interference Modulation
675
C. Rapid-Scan Fourier Spectroscopy
676
D. Summary
677
References
678
Appendix
VII
A Far-Infrared Bibliography, by E. D.
Palik
679
Author Index to Bibliogrophy
761
Index
777
|
| any_adam_object | 1 |
| author | Möller, Karl Dieter Rothschild, Walter G. |
| author_facet | Möller, Karl Dieter Rothschild, Walter G. |
| author_role | aut aut |
| author_sort | Möller, Karl Dieter |
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| dewey-full | 535/.842 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 535 - Light and related radiation |
| dewey-raw | 535/.842 |
| dewey-search | 535/.842 |
| dewey-sort | 3535 3842 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| format | Book |
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| id | DE-604.BV000931287 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T15:21:26Z |
| institution | BVB |
| isbn | 0471613134 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-000570507 |
| oclc_num | 140537 |
| open_access_boolean | |
| owner | DE-19 DE-BY-UBM DE-29T DE-91G DE-BY-TUM DE-703 DE-355 DE-BY-UBR DE-83 DE-11 DE-188 |
| owner_facet | DE-19 DE-BY-UBM DE-29T DE-91G DE-BY-TUM DE-703 DE-355 DE-BY-UBR DE-83 DE-11 DE-188 |
| physical | XIX, 797 S. Ill., graph. Darst. |
| psigel | TUB-nveb |
| publishDate | 1971 |
| publishDateSearch | 1971 |
| publishDateSort | 1971 |
| publisher | Wiley |
| record_format | marc |
| series2 | Wiley series in pure and applied optics |
| spelling | Möller, Karl Dieter Verfasser aut Far-infrared spectroscopy Karl Dieter Möller ; Walter G. Rothschild New York Wiley 1971 XIX, 797 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Wiley series in pure and applied optics Infraroodspectrometrie gtt Materia Condensada (Espectroscopia) larpcal Otica, Holografia, Laser E Cor larpcal Spectroscopie infrarouge Infrared Rays Infrared spectroscopy Spectrum Analysis Infrarotspektroskopie (DE-588)4135411-4 gnd rswk-swf Infrarotspektroskopie (DE-588)4135411-4 s DE-604 Rothschild, Walter G. Verfasser aut Digitalisierung UB Regensburg application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000570507&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Möller, Karl Dieter Rothschild, Walter G. Far-infrared spectroscopy Infraroodspectrometrie gtt Materia Condensada (Espectroscopia) larpcal Otica, Holografia, Laser E Cor larpcal Spectroscopie infrarouge Infrared Rays Infrared spectroscopy Spectrum Analysis Infrarotspektroskopie (DE-588)4135411-4 gnd |
| subject_GND | (DE-588)4135411-4 |
| title | Far-infrared spectroscopy |
| title_auth | Far-infrared spectroscopy |
| title_exact_search | Far-infrared spectroscopy |
| title_full | Far-infrared spectroscopy Karl Dieter Möller ; Walter G. Rothschild |
| title_fullStr | Far-infrared spectroscopy Karl Dieter Möller ; Walter G. Rothschild |
| title_full_unstemmed | Far-infrared spectroscopy Karl Dieter Möller ; Walter G. Rothschild |
| title_short | Far-infrared spectroscopy |
| title_sort | far infrared spectroscopy |
| topic | Infraroodspectrometrie gtt Materia Condensada (Espectroscopia) larpcal Otica, Holografia, Laser E Cor larpcal Spectroscopie infrarouge Infrared Rays Infrared spectroscopy Spectrum Analysis Infrarotspektroskopie (DE-588)4135411-4 gnd |
| topic_facet | Infraroodspectrometrie Materia Condensada (Espectroscopia) Otica, Holografia, Laser E Cor Spectroscopie infrarouge Infrared Rays Infrared spectroscopy Spectrum Analysis Infrarotspektroskopie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000570507&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT mollerkarldieter farinfraredspectroscopy AT rothschildwalterg farinfraredspectroscopy |