Structure and properties of silicate melts:
Saved in:
| Main Author: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Amsterdam [u.a.]
Elsevier
1988
|
| Series: | Developments in geochemistry
4 |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | VII, 354 S. Ill., graph. Darst. |
| ISBN: | 044442959X |
Staff View
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| 245 | 1 | 0 | |a Structure and properties of silicate melts |c B. O. Mysen |
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| adam_text | Titel: Structure and properties of silicate melts
Autor: Mysen, Bjorn O.
Jahr: 1988
TABLE OF CONTENTS
Preface...........................................................................................................................................v
Acknowledgments.......................................................................................................................ix
Chapter 1. Silica..................................................................................................................1
1.1 INTRODUCTION......................................................................................................................1
1.2 PRINCIPAL BUILDING BLOCKS AND CONCEPTS................................................................1
1.3 STRUCTURE OF S1O2...............................................................................................................4
1.3.1 Random network structure.............................................................................................5
1.3.2 Pseudocrystalline structure...........................................................................................7
1.3.3 Coexisting structures.....................................................................................................10
1.4 SUMMARY...........................................................................................................................24
Chapter 2. Metal Oxide-Silica Systems.....................................................................27
2.1 INTRODUCTION....................................................................................................................27
2.2 BULK PROPERTIES..............................................................................................................27
2.2.1 Refractive index..........................................................................................................28
2.2.2 Molar volume and compressibility...........................................................................29
2.2.3 Viscosity........................................................................................................................31
2.2.4 Entropy and heat capacity.........................................................................................37
2.3 ACTIVITY-COMPOSITION RELATIONSHIPS......................................................................39
2.3.1 Phase equilibria...........................................................................................................40
2.3.2 Thermodynamics of mixing.......................................................................................47
2.4 STRUCTURAL MODELS........................................................................................................48
2.4.1 Thermodynamic models..............................................................................................49
2.4.1.1 The Temkin model..................................................................................................50
2.4.1.2 The polymer model................................................................................................51
2.4.1.3 Multicomponent mixing and the pseudocrystalline model...........................56
2.4.2 Numerical simulation of structure...........................................................................58
2.4.2.1 Numerical calculations of local electronic structure and perturbations
from network-modifying cations.......................................................................60
2.4.2.2 Numerical simulation of anion and cation distribution................................62
2.4.3 Experimental determination of melt structure......................................................64
2.4.3.1 The anionic network structure...........................................................................64
2.4.3.2 Abundance of structural units............................................................................74
2.5 SUMMARY...........................................................................................................................77
Chapter 3. Aluminosilicate Systems.........................................................................79
3.1 INTRODUCTION....................................................................................................................79
3.2 ALUMINUM CHARGE-BALANCE........................................................................................80
¡i Table of Contents
3.3 PROPERTIES OF ALUMINOSILICATE MELTS.....................................................................80
3.3.1 Density and compressibility......................................................................................81
3.3.2 Viscosity........................................................................................................................84
3.3.3 Phase equilibria...........................................................................................................91
3.3.3.1 Activity-composition relationships...................................................................92
3.3.3.2 The pseudocrystalline model...............................................................................99
3.3.4 Thermodynamics of mixing.....................................................................................103
3.4 STRUCTURE OF ALUMINOSILICATE GLASSES AND MELTS...........................................116
3.4.1 Properties of tetrahedral bonding in aluminosilicates.....................................116
3.4.2 Structure of aluminosilicate melts and glasses at atmospheric pressure.......122
3.4.2.1 Tectosilicate melts................................................................................................124
3.4.2.2 Peralkaline aluminosilicate melts....................................................................136
3.4.2.3 Peraluminous aluminosilicate melts................................................................140
3.4.3 Structure of aluminosilicate melts at high pressure..........................................141
3.5 SUMMARY.........................................................................................................................145
Chapter 4. Iron Oxides...................................................................................................147
4.1 INTRODUCTION..................................................................................................................147
4.2 STRUCTURAL POSITIONS OF FERRIC AND FERROUS IRON IN SILICATE MELTS........148
4.3 DETERMINATION OF Fe3+/ZFe.........................................................................................155
4.4 REDOX EQUILIBRIA AND MELT STRUCTURE..................................................................157
4.4.1 Redox equilibria and extensive variables.............................................................157
4.4.2 Redox equilibria and intensive variables.............................................................164
4.5 RELATIONSHIPS BETWEEN SIMPLE AND COMPLEX SYSTEMS.....................................170
4.6 REDOX EQUILIBRIA OF IRON AND MELT POLYMERIZATION........................................172
4.7 PHASE EQUILIBRIA IN IRON-BEARING SYSTEMS........................................................176
4.8 PHYSICAL PROPERTIES OF IRON-BEARING SILICATE MELTS.....................................179
4.8.1 Volume relations........................................................................................................179
4.8.2 Viscosity of iron-bearing silicate melts................................................................182
4.9 SUMMARY.........................................................................................................................185
Chapter S. Titanium........................................................................................................187
5.1 INTRODUCTION..................................................................................................................187
5.2 PROPERTIES OF TITANIUM-BEARING SYSTEMS...........................................................188
5.3 STRUCTURAL ROLE OF TITANIUM IN MELTS AND GLASSES.......................................193
5.3.1 The system SÍO2-TÍO2.................................................................................................194
5.3.2 Titanium in depolymerized melts...........................................................................196
5.4 SUMMARY.........................................................................................................................200
Chapter 6. Phosphorous...............................................................................................201
6.1 INTRODUCTION..................................................................................................................201
Table of Contents iii
6.2 PROPERTIES OF PHOSPOROUS-BEARING SYSTEMS.......................................................201
6.3 STRUCTURAL ROLE OF PHOSPHOROUS IN SILICATE MELTS AND GLASSES...............206
6.3.1 The system SÌO2-P2O5................................................................................................206
6.3.2 Phosphorous in depolymerized melts....................................................................208
6.4 SUMMARY.........................................................................................................................215
Chapter 7. Volatiles........................................................................................................217
7.1 INTRODUCTION..................................................................................................................217
7.2 WATER................................................................................................................................219
7.3 HYDROGEN.........................................................................................................................229
7.4 SULFUR..............................................................................................................................231
7.4.1 Reduced sulfur...........................................................................................................231
7.4.2 Oxidized sulfur............................................................................................................235
7.5 CARBON..............................................................................................................................237
7.5.1 Carbon dioxide............................................................................................................238
7.5.2 Carbon monoxide.......................................................................................................243
7.5.3 Methane.......................................................................................................................244
7.6 FLUORINE...........................................................................................................................247
7.7 SUMMARY.........................................................................................................................253
Chapter 8. Multicomponent, Complex Systems..................................................255
8.1 INTRODUCTION..................................................................................................................255
8.2 DATA BASE.........................................................................................................................259
8.2.1 Bulk chemical analyses............................................................................................259
8.2.2 Structural information.............................................................................................259
8.2.2.1 Network-modifying cations...............................................................................263
8.2.2.2 Aluminum.............................................................................................................263
8.2.2.3 Ferric iron............................................................................................................266
8.2.2.4 Other cations.........................................................................................................268
8.3 STRUCTURE OF MAGMATIC LIQUIDS..............................................................................269
8.4 PETROLOGICAL IMPLICATIONS.......................................................................................279
8.4.1 Structure and properties..........................................................................................279
8.4.2 Redox equilibria and melt structure......................................................................286
8.5 SUMMARY.........................................................................................................................293
References..............................................................................................................................295
System Index..........................................................................................................................327
Subject Index.........................................................................................................................329
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| isbn | 044442959X |
| language | English |
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| series2 | Developments in geochemistry |
| spelling | Mysen, Bjorn O. Verfasser aut Structure and properties of silicate melts B. O. Mysen Amsterdam [u.a.] Elsevier 1988 VII, 354 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Developments in geochemistry 4 Minéraux silicatés Silicates Verre Glass Silicate minerals Silicatschmelze (DE-588)4181365-0 gnd rswk-swf Geochemie (DE-588)4020198-3 gnd rswk-swf Schmelze (DE-588)4130581-4 gnd rswk-swf Silicate (DE-588)4077444-2 gnd rswk-swf Silicate (DE-588)4077444-2 s Schmelze (DE-588)4130581-4 s DE-604 Geochemie (DE-588)4020198-3 s Silicatschmelze (DE-588)4181365-0 s Developments in geochemistry 4 (DE-604)BV000011334 4 HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000531535&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Mysen, Bjorn O. Structure and properties of silicate melts Developments in geochemistry Minéraux silicatés Silicates Verre Glass Silicate minerals Silicatschmelze (DE-588)4181365-0 gnd Geochemie (DE-588)4020198-3 gnd Schmelze (DE-588)4130581-4 gnd Silicate (DE-588)4077444-2 gnd |
| subject_GND | (DE-588)4181365-0 (DE-588)4020198-3 (DE-588)4130581-4 (DE-588)4077444-2 |
| title | Structure and properties of silicate melts |
| title_auth | Structure and properties of silicate melts |
| title_exact_search | Structure and properties of silicate melts |
| title_full | Structure and properties of silicate melts B. O. Mysen |
| title_fullStr | Structure and properties of silicate melts B. O. Mysen |
| title_full_unstemmed | Structure and properties of silicate melts B. O. Mysen |
| title_short | Structure and properties of silicate melts |
| title_sort | structure and properties of silicate melts |
| topic | Minéraux silicatés Silicates Verre Glass Silicate minerals Silicatschmelze (DE-588)4181365-0 gnd Geochemie (DE-588)4020198-3 gnd Schmelze (DE-588)4130581-4 gnd Silicate (DE-588)4077444-2 gnd |
| topic_facet | Minéraux silicatés Silicates Verre Glass Silicate minerals Silicatschmelze Geochemie Schmelze Silicate |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000531535&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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