Chemical processes in lakes:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
New York u.a.
Wiley
1985
|
| Schriftenreihe: | Environmental science and technology
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XX, 435 S. |
| ISBN: | 0471882615 |
| ISSN: | 0194-0287 |
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| 245 | 1 | 0 | |a Chemical processes in lakes |c ed. by Werner Stumm |
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| 650 | 4 | |a Limnologie | |
| 650 | 4 | |a Biogeochemical cycles | |
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Datensatz im Suchindex
| _version_ | 1804114724921540608 |
|---|---|
| adam_text | Titel: Chemical processes in lakes
Autor: Stumm, Werner
Jahr: 1985
CONTENTS
1. Spatial and Temporal Distribution of Chemical Substances
in Lakes: Modeling Concepts 1
Dieter M. Imboden and René P. Schwarzenbach
1. Introduction 1
2. Mass Transport in Lakes: Time and Length Scales 2
2.1. Transport Mechanisms 2
2.2. Rate Constants 6
2.3. Choice of Model 8
2.4. Box Models 9
3. One-Dimensional Vertical Model for Reactive Species
in Lakes 12
3.1. Model Structure 12
3.2. Transfer between Dissolved and Particulate Phases 13
3.3. Interaction between Sediments and Water 14
3.4. Model Equations 15
4. Application of the Model to Hydrophobie Organic
Compounds 18
4.1. Model Compounds 18
4.2. Transfer and Reaction: Rate Constants 18
4.3. Examples 20
5. Conclusions 28
References 28
2. Conceptual Models for Transport at a Redox Boundary 31
William Davison
1. Introduction 32
2. Instantaneous Concentration Profiles of Soluble
Components 33
2.1. Generalized Transport Mechanism 33
2.2. Factors Which Modify Profile Shapes 34
2.3. Water Columns 35
??
xiv Contents
2.4. Sediments 38
2.5. Sediment-Water Interfaces 39
3. Instantaneous Concentration Profiles of Participate
Components 42
3.1. Generalized Transport Mechanism 42
3.2. Water Columns 43
3.3. Sediments and the Sediment-Water Interface 44
4. General Discussion 46
5. Conclusions 48
Acknowledgments 49
References 49
3. Aqueous Surface Chemistry: Assessment of Adsorption
Characteristics of Organic Solutes by Electrochemical Methods 55
Bozena Cosovic
1. Introduction 56
2. Determination of Surface-Active Substances by
Electrochemical Methods 58
3. Surface-Active Substances in Freshwaters 61
4. Surface-Active Substances in the Sea 68
5. Interaction of Surface-Active Substances with Metals
Studied at the Electrode/Water Interface 72
6. Conclusions 76
Acknowledgments 77
References 77
4. Strategies for Microbial Resistance to Heavy Metals 81
John M. Wood and Hong Kang Wang
1. Introduction 82
2. A General Model for Metal Transport by
Microorganisms 84
3. Microbial Life in Metal-Rich Environments 86
4. Biomethylation 86
5. Intracellular Traps 88
6. The Binding of Metal Ions to Cell Surfaces
and to Extracellular Ligands 90
7. The Precipitation of Metals by the Activities of
Enzymes at the Cell Surface 92
8. Concluding Remarks 95
Acknowledgments 95
References 96
Contents xv
5. Carbon Isotopes and Productivity in the Lacustrine
and Marine Environment 99
Judith A. McKenzie
1. Introduction 100
2. Carbon Isotopes 101
3. Dissolved Inorganic Carbon 102
3.1. Lacustrine Environment 102
3.2. Marine Environment 104
4. Carbonate Precipitates 105
4.1. Lacustrine Environment 105
4.2. Marine Environment 107
5. Carbon Isotopes and Paleoproductivity 110
5.1. Lacustrine Environment 110
5.2. Marine Environment 114
6. Conclusions 116
Acknowledgments 116
References 117
6. Redox-Related Geochemistry in Lakes; Alkali Metals, Alkaline-
Earth Elements, and 137Cs 119
Edward R. Sholkovitz
1. Introduction 120
2. Biogeochemical Cycles 120
3. Fe and Mn Redox Chemistries and Cycles 121
4. Fluxes at the Sediment-Water Interface under Anoxic
Conditions 123
5. Alkali and Alkaline-Earth Elements—Distribution in
Dissolved, Suspended, and Pore-Water Phases 124
6. 137Cs in Lakes 131
6.1. General Information 131
Acknowledgments 138
References 138
7. Mechanisms Controlling the Sedimentation Sequence of Various
Elements in Prealpine Lakes 143
Hans-Henning Stabel
1. Introduction 144
2. Analysis of Sedimentation Processes 145
2.1. Sources, Fluxes, and Chemical Composition
of Paniculate Matter 145
2.2. Seasonality of Elemental Fluxes 149
2.3. Stoichiometric Relations in the Organic Material 161
xvi Contents
3. Conclusions 163
References 164
8. The Pavin Crater Lake 169
Jean-Marie Martin
1. Introduction 169
2. The Environmental Framework 170
2.1. The Water Balance 170
2.2. The Chemical Functioning 173
2.3. Sedimentation Rate and Pavin Lake History 175
3. Atmospheric Deposition of Pollutants 179
3.1. Trace Metals 179
3.2. Artificial Radionuclides 181
4. Conclusions 184
Acknowledgments 185
References 185
9. Phosphate Interactions at the Sediment-Water Interface 189
Peter Boccini
1. Introduction 190
2. Concepts and Methodology 191
3. Phenomenology of Phosphorus Transport Processes 192
3.1. Chemical Characteristics of the Solid Phase 192
3.2. Seasonal and Spatial Variation of the Chemical
Composition of Pore Waters 194
3.3. Phosphate and Manganese Fluxes at the Sediment
Boundary Layer 195
4. A Two-Box Model for the Sediment Boundary Layer 198
4.1. Structure and Biochemical Properties of the
Boundary Layer 198
4.2. Modeling the Dynamics of Phosphorus Transport 201
5. Conclusions 201
6. Appendix 202
6.1. Sampling Locations, Separation Techniques, and
Chemical Analysis 202
6.2. Flux Measurements Across the Sediment
Boundary Layer 202
References 204
10. The Influence of Coagulation and Sedimentation on the Fate
of Particles, Associated Pollutants, and Nutrients in Lakes 207
Charles R. O Melia
1. Introduction 207
2. The Model 208
Contents xvii
3. Previous Work 213
4. Results 213
4.1. Colloidal Stability 214
4.2. Kinetics 219
4.3. Sorbed Subtances 220
5. Discussion 220
6. Conclusions 223
Acknowledgments 223
References 224
11. The Coupling of Elemental Cycles by Organisms: Evidence
from Whole-Lake Chemical Perturbations 225
David W. Schindler
1. Introduction 226
2. Consequences of Altering the Input of Nutrients 226
3. Changes Induced by Addition of Phosphorus 228
4. Changes Induced by Addition of Nitrogen 233
5. Consequences of Altering the Input of Sulfate 235
6. Multiple Linkages between Cycles 240
7. Key Sites for the Organisms Which Couple Geochemical
Cycles 241
8. How Robust Are the Biological Coupling Mechanisms? 244
9. Conclusions 245
Acknowledgments 246
References 246
12. The Geobiological Cycle of Trace Elements in Aquatic Systems:
Redfield Revisited 251
François M. M. Morel and Robert J. M. Hudson
1. Introduction 251
2. The Nature of the Scavenging Phase 253
3. Metal Uptake by Algae 260
4. Metal Concentrations in Oceanic Particles (A
Teleological Rationalization) 265
5. Conclusion 269
6. Appendix: Metal Partitioning and Oceanic Residence
Time 271
6.1. Metal Residence Times 272
6.2. Particle Residence Times 274
6.3. Estimates of Partitioning 274
6.4. Partitioning onto Model Solids 274
7. Summary 277
Acknowledgments 278
References 278
xviii Contents
13. Metal Transfer Mechanisms in Lakes; The Role of Settling
Particles 283
Laura Sigg
1. Introduction 283
2. Important Factors Regulating the Heavy-Metal
Concentrations in Lakes 285
2.1. Speciation and Partition of Metals between
Solution and Solid Phase 285
2.2. Metal Uptake by Phytoplankton 288
2.3. Redox Processes 298
2.4. Precipitation of Solid Phases 300
2.5. Quantitative Description of the Distribution of
Heavy Metals between Dissolved and Particulate
Phase 300
3. Mass Balances, Residence Times, and Steady State 303
4. Comparison of Heavy-Metal Cycles in Oceans and
Lakes 305
5. Conclusions 306
Acknowledgments 307
References 307
14. Acidification of Aquatic and Terrestrial Systems 311
Jer aid L. Schnoor and Werner Stumm
1. Introduction 312
2. Genesis of Acid Precipitation 313
3. Acid- or Base-Neutralizing Capacity 316
4. Processes Affecting Acid-Neutralizing Capacity (ANC) 320
4.1. ANC of Soil 320
4.2. Chemical Weathering 320
4.3. Aluminum Dissolution 323
4.4. Biomass Synthesis 325
4.5. Redox Processes 327
5. Lake Response 328
5.1. Trickle-Down Model 329
5.2. Evaluation of Coefficients 331
5.3. Time to Steady State 332
6. Summary 335
Acknowledgments 336
References 336
15. The Chemistry of Bog Waters 339
Evilk Gorham, Steven J. Eisenreich, Jesse Ford,
and Mary V. Santelmann
1. Introduction 339
1.1. Early Work on the Chemistry of Bog Waters 343
Contents XIX
1.2. The 1940s through the 1960s 344
1.3. The Present Study 345
2. Methods 345
2.1. Choice of Sites 345
2.2. Sample Collection, Treatment, and Storage 347
2.3. Analysis 348
3. Environmental Controls on the Chemistry of Bog Waters 349
3.1. Sea Spray 350
3.2. Dustfall from Blown Soil 350
3.3. Air Pollution 352
3.4. Climate 354
4. Comparative Chemistry of Bog Waters from Different
Regions 355
5. The Acidity of Bog Waters 356
6. Concluding Remarks 360
7. Acknowledgments 361
References 361
16. Lake Restoration 363
René Gächter and Dieter M. Imboden
1. Introduction: Lake Eutrophication, An Unsolved
Problem 365
2. A Simple Model for Lake Restoration 367
3. Nonlinear and Nonstationary Behavior of Phosphorus
Concentration in Lakes 370
4. Lake Restoration by Oxygen Input 375
4.1. Artificial Mixing 375
4.2. Artificial Oxygen Input 377
5. Diversion of Hypolimnic Water 380
5.1. Change of the Permissible Phosphorus Loading
Due to Hypolimnic Diversion (HD) 381
5.2. Influence of Hypolimnic Diversion on the
Oxygen Balance 383
5.3. Examples of Hypolimnic Diversion 384
6. Summary and Conclusions 386
References 387
17. Kinetics of Chemical Processes of Importance in Lacustrine
Environments 389
James J. Morgan and Alan T. Stone
1. Introduction 390
2. Physical and Chemical Rates 391
3. Characteristic Time Scales 394
4. Aqueous Chemical Kinetics 396
4.1. Phenomenological Description of Reaction Rates 396
xx Contents
4.2. Reaction Mechanisms 397
4.3. Theories of Elementary Reactions 398
5. Activated Complex Theory 399
6. Arrhenius Equation and Parameters 402
7. Slow Elementary Reactions 403
8. Examples of Elementary Aqueous Reactions 405
9. Rapid Aqueous Reactions 409
9.1. Coordination 409
9.2. Redox Intermediates 409
10. Ionic Strength and Elementary Reactions 410
11. Complex Reactions 411
11.1. Formulation of the Rate 411
11.2. Reversible Reactions 412
11.3. Reversible and Irreversible Reaction Sequences 414
11.4. Concurrent Reactions 417
11.5. Radical and Chain Reaction Mechanisms 418
12. Importance of pH in Aqueous Kinetics 420
13. A Concluding Kinetic Overview 422
Acknowledgments 424
References 424
Index 427
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| spelling | Chemical processes in lakes ed. by Werner Stumm New York u.a. Wiley 1985 XX, 435 S. txt rdacontent n rdamedia nc rdacarrier Environmental science and technology 0194-0287 Cycles biogéochimiques Eau - Chimie Lacs Limnologie Biogeochemical cycles Lakes Limnology Water chemistry Chemie (DE-588)4009816-3 gnd rswk-swf Hydrochemie (DE-588)4072678-2 gnd rswk-swf Limnologie (DE-588)4035769-7 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Limnologie (DE-588)4035769-7 s Chemie (DE-588)4009816-3 s DE-604 Hydrochemie (DE-588)4072678-2 s Stumm, Werner 1924-1999 Sonstige (DE-588)140381414 oth HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000156411&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Chemical processes in lakes Cycles biogéochimiques Eau - Chimie Lacs Limnologie Biogeochemical cycles Lakes Limnology Water chemistry Chemie (DE-588)4009816-3 gnd Hydrochemie (DE-588)4072678-2 gnd Limnologie (DE-588)4035769-7 gnd |
| subject_GND | (DE-588)4009816-3 (DE-588)4072678-2 (DE-588)4035769-7 (DE-588)4143413-4 |
| title | Chemical processes in lakes |
| title_auth | Chemical processes in lakes |
| title_exact_search | Chemical processes in lakes |
| title_full | Chemical processes in lakes ed. by Werner Stumm |
| title_fullStr | Chemical processes in lakes ed. by Werner Stumm |
| title_full_unstemmed | Chemical processes in lakes ed. by Werner Stumm |
| title_short | Chemical processes in lakes |
| title_sort | chemical processes in lakes |
| topic | Cycles biogéochimiques Eau - Chimie Lacs Limnologie Biogeochemical cycles Lakes Limnology Water chemistry Chemie (DE-588)4009816-3 gnd Hydrochemie (DE-588)4072678-2 gnd Limnologie (DE-588)4035769-7 gnd |
| topic_facet | Cycles biogéochimiques Eau - Chimie Lacs Limnologie Biogeochemical cycles Lakes Limnology Water chemistry Chemie Hydrochemie Aufsatzsammlung |
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