Towards molecular photocatalysts for overall water splitting:
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| Format: | Abschlussarbeit Buch |
| Sprache: | English |
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Ulm
2014
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| Online-Zugang: | Inhaltsverzeichnis Inhaltsverzeichnis |
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| Beschreibung: | 233 Blätter Diagramme 30 cm |
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Datensatz im Suchindex
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QLI 30^
ULM UNIVERSITY UNIVERSITAT
TOWARDS MOLECULAR PHOTOCATALYSTS FOR
OVERALL WATER SPLITTING
DISSERTATION ZUR ERLANGUNG DES DOKTORGRADES DR.RER.NAT.
DER FAKULTAT FUR NATURWISSENSCHAFTEN DER UNIVERSITAT ULM
VORGELEGT VON
DIPLOMCHEMIKER ROBERT OLIVER STAEHLE
GEBOREN AM 25.07.1984 IN STUTTGART
2014
HTTP://D-NB.INFO/1059371332
TABLE OF CONTENT
1. MOTIVATION 1
2. STATE OF THE ART 4
3. SCOPE OF THE THESIS 31
4. INVESTIGATED SYSTEMS 33
4.1. INFLUENCE OF PLANAR AROMATIC ORGANIC MOLECULES ON THE CATALYTIC
PERFORMANCE 33
4.2. WATER REDUCTION IN THE PRESENCE OF OXYGEN 36
4.2.1. MECHANISTIC STUDIES 36
4.2.2. MODIFICATION OF THE CHROMOPHORE 41
4.3. CARBENES IN THE CATALYTIC WATER SPLITTING 43
4.3.1. INTRAMOLECULAR SYSTEMS CONTAINING N-HETEROCYCLIC CARBENES 43
4.3.2. INTERMOLECULAR SYSTEMS - MODIFICATIONS OF THE CHROMOPHORE 46
4.3.2.1. MODIFICATION OF THE PHENANTHROLINE BACKBONE 46
4.3.2.2. MODIFICATION OF THE N-HETEROCYCLIC CARBENE UNIT 47
4.3.2.3. MODIFICATION OF THE TERMINAL LIGANDS 49
4.3.2.4. CATALYTIC ACTIVITY OF MODIFIED COMPLEXES 54
4.3.2.5. MODIFICATION OF THE METAL CENTRE 58
5. SUMMARY AND OUTLOOK 60
6. REFERENCES 63
T
7. PUBLICATIONS 67
7.1. [RSI]: SUPRAMOLECULAR ACTIVATION OF A MOLECULAR PHOTOCATALYST 68
7.2. [RS2]: PHOTOCATALYTIC GENERATION OF HYDROGEN FROM WATER UNDER
AEROBIC CONDITIONS 95
7.3. [RS3]: AN IMPROVED SYNTHESIS OF 4-CYANO-L,10-PHENANTHROLINE,
4,7-DICYANO-L
5
10-
PHENANTHROLINE AND THEIR BIS (4,4'-DI-TERT-BUTYL-2
S
2'-BIPYRIDINE)RUTHENIUM(IL)
COMPLEXES 109
7.4. [RS4]: CARBENE BASED PHOTOCHEMICAL MOLECULAR ASSEMBLIES FOR SOLAR
DRIVEN HYDROGEN
GENERATION 130
7.5. [RS5]: IMPROVED OXYGEN RESISTANCE IN RUTHENIUM PHOTOCENTRES BY
LIGAND DESIGN. 178
7.6. [RS6]: WATER OXIDATION CATALYZED BY MONONUCLEAR RUTHENIUM COMPLEXES
WITH A 2,2'-
BIPYRIDINE-6,6'-DICARBOXYLATE (BDA) LIGAND: HOW LIGAND ENVIRONMENT
INFLUENCES
THE CATALYTIC BEHAVIOR 194
8. CURRICULUM VITAE 231
9. PUBLICATIONS AND CONFERENCE CONTRIBUTIONS 232
9.1. PUBLICATIONS IN PEER REVIEWED JOURNALS 232
9.2. SPECIALIST BOOKS 232
9.3. CONFERENCE PROCEEDINGS 232
9.3.1. ORAL PRESENTATIONS 232
9.3.2. POSTER CONTRIBUTIONS 233
10. ABBREVIATIONS 234
11. ACKNOWLEDGMENTS 237
12. DECLARATION OF HONESTY IN ACADEMIC WORK 238 |
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| spelling | Staehle, Robert Oliver 1984- Verfasser (DE-588)1059652714 aut Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle Ulm 2014 233 Blätter Diagramme 30 cm txt rdacontent n rdamedia nc rdacarrier Enthällt Sonderabdrucke Dissertation Universität Ulm 2014 Wasserstofferzeugung (DE-588)4189271-9 gnd rswk-swf Fotokatalyse (DE-588)4193873-2 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Wasserstofferzeugung (DE-588)4189271-9 s Fotokatalyse (DE-588)4193873-2 s DE-604 B:DE-101 application/pdf http://d-nb.info/1059371332/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=031256151&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Staehle, Robert Oliver 1984- Towards molecular photocatalysts for overall water splitting Wasserstofferzeugung (DE-588)4189271-9 gnd Fotokatalyse (DE-588)4193873-2 gnd |
| subject_GND | (DE-588)4189271-9 (DE-588)4193873-2 (DE-588)4113937-9 |
| title | Towards molecular photocatalysts for overall water splitting |
| title_auth | Towards molecular photocatalysts for overall water splitting |
| title_exact_search | Towards molecular photocatalysts for overall water splitting |
| title_full | Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle |
| title_fullStr | Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle |
| title_full_unstemmed | Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle |
| title_short | Towards molecular photocatalysts for overall water splitting |
| title_sort | towards molecular photocatalysts for overall water splitting |
| topic | Wasserstofferzeugung (DE-588)4189271-9 gnd Fotokatalyse (DE-588)4193873-2 gnd |
| topic_facet | Wasserstofferzeugung Fotokatalyse Hochschulschrift |
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