Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics:
Gespeichert in:
| 1. Verfasser: | |
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| Format: | Abschlussarbeit Buch |
| Sprache: | English |
| Veröffentlicht: |
2013
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| Schlagworte: | |
| Online-Zugang: | kostenfrei Inhaltsverzeichnis |
| Beschreibung: | Zsfassung in dt. und engl. Sprache |
| Beschreibung: | 127 S. graph. Darst. |
Internformat
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| 245 | 1 | 0 | |a Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics |c von Friedrich Andreas Sperlich |
| 246 | 1 | 3 | |a Elektron-Paramagnetische Resonanz-Spektroskopie von konjugierten Polymeren und Fullerenen für die organische Photovoltaik |
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Datensatz im Suchindex
| _version_ | 1804151491923017728 |
|---|---|
| adam_text | CONTENTS
1 INTRODUCTION 5
2 ORGANIC SEMICONDUCTORS FOR PHOTOVOLTAICS 9
2.1 ORGANIC SEMICONDUCTORS 9
2.2 EXCITED SINGLET AND TRIPLET STATES 10
2.3 ORGANIC SOLAR CELLS 11
2.4 USED MATERIALS 13
3 ELECTRON PARAMAGNETIC RESONANCE 17
3.1 ZEEMAN SPLITTING 17
3.2 SPIN-I
/2
SYSTEMS 18
3.2.1 THE G-FACTOR AND EPR POWDER SPECTRA 19
3.2.2 LINE BROADENING 20
3.3 HIGH-FREQUENCY EPR 23
3.4 ELECTRON-ELECTRON INTERACTIONS 25
3.4.1 THE ANISOTROPIC DIPOLE-DIPOLE INTERACTION - D 25
3.4.2 THE ISOTROPIC EXCHANGE INTERACTION - / 27
3.4.3 EIGENSTATES AND BASE TRANSFORMATIONS 28
3.5 SPIN-COUPLED RADICAL PAIRS 32
3.6 TRIPLET EXCITONS 34
3.7 POLARON PAIRS 37
3.8 OPTICALLY DETECTED MAGNETIC RESONANCE 37
4 EXPERIMENTAL SECTION 41
4.1 SAMPLE PREPARATION 41
4.2 THE X-BAND EPR
SPECTROMETER 41
4.2.1 CONTINUOUS WAVE EPR 43
4.2.2 TIME-RESOLVED EPR 44
4.2.3 OPTICALLY DETECTED MAGNETIC RESONACE 45
4.3 PHOTO-INDUCED ABSORPTION-PIA 46
3
HTTP://D-NB.INFO/1044048794
CONTENTS
5 RESULTS 49
5.1 SPECTROSCOPIC SIGNATURES OF PHOTO-GENERATED
CYO
-FULLERENE RADICAL ANIONS 49
5.1.1 INTRODUCTION 50
5.1.2 EXPERIMENTAL DETAILS 51
5.1.3 RESULTS 52
5.1.4 DISCUSSION 60
5.1.5 CONCLUSION 62
5.2 CT IN POLYMER:PC6OBM:PC7OBM TERNARY BLENDS: WHICH FULLERENE GETS
THE ELECTRON? 63
5.2.1 INTRODUCTION 64
5.2.2 EXPERIMENTAL DETAILS 66
5.2.3 RESULTS 68
5.2.4 DISCUSSION 76
5.2.5 CONCLUSION 76
5.3 (IR-)
REVERSIBLE P3HT:02 INTERACTIONS STUDIED BY SPIN-SENSITIVE METHODS . 79
5.3.1 INTRODUCTION 80
5.3.2 EXPERIMENTAL DETAILS 80
5.3.3 RESULTS 82
5.3.4 DISCUSSION 90
5.3.5 CONCLUSION 92
5.4 TEMPERATURE-DEPENDENT CHARGE SEPARATION DYNAMICS IN P3HT
:PC6OBM
. 93
5.4.1 INTRODUCTION 94
5.4.2 EXPERIMENTAL DETAILS 95
5.4.3 RESULTS AND DISCUSSION 95
5.4.4 CONCLUSION 101
6 SUMMARY 103
BIBLIOGRAPHY 108
7 APPENDIX 121
7.1 LIST OF USEFUL CONSTANTS 121
7.2 PUBLICATIONS AND CONFERENCE CONTRIBUTIONS 122
7.3 LEBENSLAUF 126
7.4 DANKSAGUNG 127
4
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| discipline | Chemie / Pharmazie Physik Energietechnik |
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| indexdate | 2024-07-10T00:55:40Z |
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| spelling | Sperlich, Andreas 1981- Verfasser (DE-588)104359213X aut Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics von Friedrich Andreas Sperlich Elektron-Paramagnetische Resonanz-Spektroskopie von konjugierten Polymeren und Fullerenen für die organische Photovoltaik 2013 127 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Zsfassung in dt. und engl. Sprache Würzburg, Univ., Diss., 2013 Organischer Halbleiter (DE-588)4172780-0 gnd rswk-swf Fotovoltaik (DE-588)4121476-6 gnd rswk-swf Organische Solarzelle (DE-588)7617672-1 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Organische Solarzelle (DE-588)7617672-1 s DE-604 Fotovoltaik (DE-588)4121476-6 s Organischer Halbleiter (DE-588)4172780-0 s Erscheint auch als Online-Ausgabe urn:nbn:de:bvb:20-opus-81244 https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-81244 Resolving-System kostenfrei Volltext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026839310&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Sperlich, Andreas 1981- Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics Organischer Halbleiter (DE-588)4172780-0 gnd Fotovoltaik (DE-588)4121476-6 gnd Organische Solarzelle (DE-588)7617672-1 gnd |
| subject_GND | (DE-588)4172780-0 (DE-588)4121476-6 (DE-588)7617672-1 (DE-588)4113937-9 |
| title | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics |
| title_alt | Elektron-Paramagnetische Resonanz-Spektroskopie von konjugierten Polymeren und Fullerenen für die organische Photovoltaik |
| title_auth | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics |
| title_exact_search | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics |
| title_full | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics von Friedrich Andreas Sperlich |
| title_fullStr | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics von Friedrich Andreas Sperlich |
| title_full_unstemmed | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics von Friedrich Andreas Sperlich |
| title_short | Electron Paramagnetic Resonance Spectroscopy of Conjugated Polymers and Fullerenes for Organic Photovoltaics |
| title_sort | electron paramagnetic resonance spectroscopy of conjugated polymers and fullerenes for organic photovoltaics |
| topic | Organischer Halbleiter (DE-588)4172780-0 gnd Fotovoltaik (DE-588)4121476-6 gnd Organische Solarzelle (DE-588)7617672-1 gnd |
| topic_facet | Organischer Halbleiter Fotovoltaik Organische Solarzelle Hochschulschrift |
| url | https://nbn-resolving.org/urn:nbn:de:bvb:20-opus-81244 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026839310&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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