Reaction mechanisms in carbon dioxide conversion:
Gespeichert in:
| Hauptverfasser: | , , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin ; Heidelberg
Springer
[2016]
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis Inhaltsverzeichnis |
| Beschreibung: | xviii, 409 Seiten Illustrationen, Diagramme, Portraits (teilweise farbig) |
| ISBN: | 9783662468302 3662468301 |
Internformat
MARC
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| 245 | 1 | 0 | |a Reaction mechanisms in carbon dioxide conversion |c Michele Aresta, Angela Dibenedetto, Eugenio Quaranta |
| 264 | 1 | |a Berlin ; Heidelberg |b Springer |c [2016] | |
| 264 | 4 | |c © 2016 | |
| 300 | |a xviii, 409 Seiten |b Illustrationen, Diagramme, Portraits (teilweise farbig) | ||
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| 650 | 0 | 7 | |a Präparative organische Chemie |0 (DE-588)4121505-9 |2 gnd |9 rswk-swf |
| 653 | |a Carbon dioxide molecular orbitals | ||
| 653 | |a CO2 spectroscopic techniques | ||
| 653 | |a CO2 enzymatic conversion | ||
| 653 | |a CO2 coordination to metal centres | ||
| 653 | |a CO2 insertion into 11-X | ||
| 653 | |a CO2 electrochemical reduction | ||
| 653 | |a CO2 photocatalytic reduction | ||
| 653 | |a Chemie/Organische Chemie | ||
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Datensatz im Suchindex
| _version_ | 1804176053289091072 |
|---|---|
| adam_text | CONTENTS
1 THE CARBON DIOXIDE MOLECULE 1
1.1 INTRODUCTION 1
1.2 ELECTRONIC PROPERTIES OF C0
2
2
1.2.1 GROUND STATE OF CARBON DIOXIDE 2
1.2.2 LOWEST EXCITED STATES OF CARBON DIOXIDE 6
1.3 MAIN FEATURES OF CARBON DIOXIDE REACTIVITY 8
1.3.1 CARBON DIOXIDE AS O-NUCLEOPHILE 9
1.3.2 CARBON DIOXIDE AS C-ELECTROPHILE 10
1.3.3 AMPHOTERIC REACTIVITY OF CARBON DIOXIDE 11
1.4 CARBON DIOXIDE RADICAL ANION, C0
2
~ 12
1.5 CARBON DIOXIDE RADICAL CATION, C0
2+
19
1.6 SPECTROSCOPIC TECHNIQUES APPLIED TO THE C0
2
STATES 20
1.6.1 IR SPECTROSCOPY 20
1.6.2 UV SPECTRUM OF CARBON DIOXIDE 22
1.6.3 NUCLEAR MAGNETIC RESONANCE (NMR) SPECTROSCOPY ... 26
REFERENCES 27
2 C0
2
COORDINATION TO METAL CENTRES: MODES OF BONDING AND
REACTIVITY 35
2.1 MODE OF BONDING OF CARBON DIOXIDE TO TRANSITION-METAL
CENTRES 35
2.2 XRD STRUCTURE OF R|
2
-C,0 MONONUCLEAR METAL COMPLEXES 37
2.3 XRD STRUCTURAL DATA FOR RI -C METAL COMPLEXES 41
2.4 XRD STRUCTURAL CHARACTERIZATION OF O-END-ON COMPLEXES .... 43
2.5 MULTINUCLEAR COMPLEXES 43
2.5.1 SIDE-ON BONDED COMPLEXES 43
2.5.2 O-END-ON BONDED COMPLEXES 44
2.6 SPECTROSCOPIC (IR AND
13
C-NMR) DATA FOR THE COMPLEXES
CORRELATED TO THE VARIOUS MODES OF BONDING OF C0
2
47
2.6.1 INFRARED DATA RELEVANT TO TRANSITION METAL
COMPLEXES 47
XI
HTTP://D-NB.INFO/1068076755
XII
CONTENTS
2.6.2 NMR DATA FOR TRANSITION METAL COMPLEXES 49
2.7 FLUXIONALITY OF THE C0
2
MOLECULE COORDINATED TO TRANSITION
METAL SYSTEMS 51
2.8 INTERACTION OF C0
2
WITH METAL ATOMS IN LOW-TEMPERATURE
SOLID-INERT-GAS MATRICES 55
2.9 INTERACTION OF METAL CATIONS WITH C0
2
IN THE GAS PHASE 57
2.10 REACTIONS OF COORDINATED C0
2
58
2.10.1 REACTION OF COORDINATED C0
2
WITH ELECTROPHILES AND
O-TRANSFER FROM C0
2
TO PRODUCE CO 59
2.10.2 REACTIONS OF COORDINATED C0
2
WITH NUCLEOPHILES. ... 63
2.11 CONCLUSIONS 64
REFERENCES 64
3 INTERACTION OF C0
2
WITH ELECTRON-RICH MOIETIES 71
3.1 REACTION WITH THE HYDRIDE ION 71
3.2 REACTION WITH HYDROXIDE AND ALKOXIDE SPECIES 72
3.3 REACTION WITH CARBANIONS 73
3.4 REACTION WITH AMINES 74
REFERENCES 82
4 INSERTION OF C0
2
INTO E-X BONDS 85
4.1 CARBON DIOXIDE INSERTION INTO M-H BONDS 85
4.2 C0
2
INSERTION INTO M-OH BONDS 91
4.3 C0
2
INSERTION INTO M-C BONDS 95
4.4 C0
2
INSERTION INTO M-OR BONDS 97
4.5 INSERTION INTO M-0
2
BONDS 98
4.6 C0
2
INSERTION INTO M-N BONDS 102
4.6.1 INSERTION INTO TRANSITION METAL AMIDES 102
4.6.2 INSERTION INTO MAIN GROUP AND POST-TRANSITION METAL
AMIDES 108
4.6.3 INSERTION INTO AMIDES OF NON-METALLIC ELEMENTS 112
4.7 C0
2
INSERTION INTO M-P BONDS 115
4.8 C0
2
INSERTION INTO C-C BONDS 117
4.9 C0
2
INSERTION INTO C-N BONDS 120
4.10 INSERTION INTO OTHER E-X BONDS 127
4.10.1 INSERTION INTO M-M BONDS 127
4.10.2 INSERTION INTO SI-H BONDS 128
4.10.3 INSERTION INTO C-H BONDS 129
4.11 CONCLUSIONS 131
REFERENCES 131
5 INTERACTION OF C0
2
WITH C-C MULTIPLE BONDS 143
5.1 INTRODUCTION 143
5.2 OXIDATIVE COUPLING WITH C0
2
144
5.3 CARBOXYLATION OF OLEFINS 147
5.4 CARBOXYLATION OF ALKYNES 156
CONTENTS XIII
5.5 CARBOXYLATION OF ALLENES 164
5.6 CARBOXYLATION OF CONJUGATED DIEIIES 169
REFERENCES 176
6 REACTION MECHANISMS IN THE DIRECT CARBOXYLATION OF ALCOHOLS,
POLYOLS, CYCLIC ETHERS, AND CYCLIC AMINES TO AFFORD MONOMERIC
COMPOUNDS AND POLYMERIC MATERIALS 183
6.1 UTILIZATION OF ORGANIC CARBONATES AND CONVENTIONAL SYNTHETIC
ROUTES 183
6.2 DIRECT CARBOXYLATION OF ALCOHOLS 185
6.2.1 THERMODYNAMIC AND KINETIC ISSUES 185
6.2.2 REACTION MECHANISM 187
6.3 DIRECT CARBOXYLATION OF DIOLS AND POLYOLS 210
6.4 OXIDATIVE CARBOXYLATION OF OLEFINS TO AFFORD CYCLIC
CARBONATES 213
6.5 CARBOXYLATION OF CYCLIC ETHERS 216
6.5.1 SYNTHESIS OF MONOMELIC CYCLIC CARBONATES 217
6.5.2 SYNTHESIS OF POLYCARBONATES 221
6.6 FORMATION OF POLYURETHANES: CARBOXYLATION OF CYCLIC
AMINES 223
6.7 CONCLUSIONS 225
REFERENCES 226
7 CARBON DIOXIDE CONVERSION IN HIGH TEMPERATURE REACTIONS 237
7.1 INTRODUCTION 237
7.2 C0
2
AS OXIDANT 238
7.2.1 OCM PROMOTED BY C0
2
238
7.2.2 OXIDATIVE DEHYDROGENATION OF ALKANES 243
7.2.3 OXIDATIVE DEHYDROGENATION OF ETHYLBENZENE TO
STYRENE 254
7.2.4 C0
2
(DRY) REFORMING OF METHANE 265
7.3 HYDROGENATION OF C0
2
277
7.3.1 REVERSE WATER GAS SHIFT REACTION (RWGS) 278
7.3.2 C0
2
HYDROGENATION TO METHANOL AND DME 278
7.3.3 CATALYTIC SYSTEMS FOR C0
2
HYDROGENATION 280
7.3.4 REACTION MECHANISM FOR C0
2
HYDROGENATION 285
7.4 CONCLUSIONS 295
REFERENCES 296
8 ONE- AND MULTI-ELECTRON PATHWAYS FOR THE REDUCTION OF C0
2
INTO CI
AND C1+ ENERGY-RICHER MOLECULES: SOME THERMODYNAMIC AND
KINETIC FACTS 311
8.1 INTRODUCTION 311
8.2 KEY STEPS AND ASPECTS IN C0
2
REDUCTION 312
8.3 ONE-ELECTRON TRANSFER TO C0
2
VS MULTI-ELECTRON TRANSFER 321
XIV
CONTENTS
8.4 COMPETITIVE COORDINATION OF C0
2
AND H
+
TO A CATALYTIC CENTRE
AND THEIR REDUCTION 322
8.5 SEQUENTIAL ONE-ELECTRON PLUS ONE-PROTON PATHWAYS IN
MULTI-ELECTRON REDUCTION OF BOUND CO2 326
8.6 PHOTOCHEMICAL AND PHOTOELECTROCHEMICAL REDUCTION OF C0
2
. . . 332
8.7 PERSPECTIVE ELECTROCHEMICAL, PHOTOCHEMICAL AND
PHOTOELECTROCHEMICAL REDUCTION OF CO2 339
REFERENCES 340
9 ENZYMATIC CONVERSION OF C0
2
(CARBOXYLATION REACTIONS AND
REDUCTION TO ENERGY-RICH CI MOLECULES) 347
9.1 INTRODUCTION 347
9.2 C0
2
FIXATION IN BIOSYNTHESIS 348
9.2.1 CALVIN-BENSON-BASSHAM-CYCLE 349
9.2.2 REDUCTIVE TCA (ARNON-BUCHANAN) CYCLE 350
9.2.3 REDUCTIVE ACETYL-COA (WOOD-LJUNGDAHL)
PATHWAY 350
9.2.4 ACYL-COA CARBOXYLATION PATHWAYS 351
9.3 CARBOXYLATION REACTIONS 353
9.3.1 BIO-CARBOXYLATION OF AROMATIC AND HETERO-AROMATIC
COMPOUNDS 353
9.3.2 BIO-CARBOXYLATION OF EPOXIDES 357
9.4 REDUCTION REACTIONS 358
9.4.1 CARBON MONOXIDE DEHYDROGENASES 358
9.4.2 FORMATE DEHYDROGENASES 360
9.4.3 FORMALDEHYDE DEHYDROGENASE 360
9.4.4 ALCOHOL DEHYDROGENASES 361
9.4.5 PRODUCTION OF ACETIC ACID 361
9.4.6 REDUCTION OF C0
2
TO CARBON MONOXIDE OR FORMATE. . . 362
9.4.7 BYCONVERSION OF CARBON DIOXIDE INTO METHANOL 364
REFERENCES 366
10 THERMODYNAMICS AND APPLICATIONS OF C0
2
HYDRATES 373
10.1 INTRODUCTION 373
10.2 STRUCTURE OF GAS HYDRATES 376
10.2.1 FORMATION OF GAS HYDRATES FROM A MICROSCOPIC
PERSPECTIVE 376
10.2.2 CRYSTAL STRUCTURES OF GAS HYDRATES 378
10.2.3 CHARACTERISTICS OF C0
2
HYDRATES 381
10.3 PHYSICAL PROPERTIES OF C0
2
HYDRATES 382
10.3.1 MECHANICAL PROPERTIES 384
10.3.2 THERMAL PROPERTIES 384
10.3.3 OTHER PHYSICAL PROPERTIES 386
10.4 PHASE EQUILIBRIUM OF C0
2
HYDRATE 386
CONTENTS XV
10.4.1 EXPERIMENTAL METHODS TO STUDY HYDRATE PHASE
EQUILIBRIA 386
10.4.2 PRESSURE-TEMPERATURE PHASE DIAGRAM OF C0
2
+ H
2
0
SYSTEM 389
10.5 APPLICATIONS OF C0
2
HYDRATES 390
10.5.1 FORMATION OF C0
2
HYDRATE 390
10.5.2 DISSOCIATION OF C0
2
HYDRATE 39-1
10.5.3 C0
2
CAPTURE AND SEQUESTRATION 392
10.5.4 REPLACEMENT OF CH
4
BY C0
2
IN NATURALLY OCCURRING
HYDRATES 395
10.5.5 C0
2
HYDRATES IN REFRIGERATION PROCESSES 396
REFERENCES 399
INDEX 403
|
| any_adam_object | 1 |
| author | Aresta, Michele 1940- Dibenedetto, Angela 1968- Quaranta, Eugenio 1957- |
| author_GND | (DE-588)1059262282 (DE-588)1043471332 (DE-588)1142397882 |
| author_facet | Aresta, Michele 1940- Dibenedetto, Angela 1968- Quaranta, Eugenio 1957- |
| author_role | aut aut aut |
| author_sort | Aresta, Michele 1940- |
| author_variant | m a ma a d ad e q eq |
| building | Verbundindex |
| bvnumber | BV043446631 |
| classification_rvk | VH 6000 VK 6000 |
| ctrlnum | (OCoLC)936806491 (DE-599)DNB1068076755 |
| dewey-full | 547.2 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 547 - Organic chemistry |
| dewey-raw | 547.2 |
| dewey-search | 547.2 |
| dewey-sort | 3547.2 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| format | Book |
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| id | DE-604.BV043446631 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T07:26:04Z |
| institution | BVB |
| isbn | 9783662468302 3662468301 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-028864143 |
| oclc_num | 936806491 |
| open_access_boolean | |
| owner | DE-29T DE-11 |
| owner_facet | DE-29T DE-11 |
| physical | xviii, 409 Seiten Illustrationen, Diagramme, Portraits (teilweise farbig) |
| publishDate | 2016 |
| publishDateSearch | 2016 |
| publishDateSort | 2016 |
| publisher | Springer |
| record_format | marc |
| spelling | Aresta, Michele 1940- Verfasser (DE-588)1059262282 aut Reaction mechanisms in carbon dioxide conversion Michele Aresta, Angela Dibenedetto, Eugenio Quaranta Berlin ; Heidelberg Springer [2016] © 2016 xviii, 409 Seiten Illustrationen, Diagramme, Portraits (teilweise farbig) txt rdacontent n rdamedia nc rdacarrier Reaktivität (DE-588)4208182-8 gnd rswk-swf Kohlendioxid (DE-588)4031648-8 gnd rswk-swf Reaktionsmechanismus (DE-588)4177123-0 gnd rswk-swf Ausgangsmaterial (DE-588)4143518-7 gnd rswk-swf Präparative organische Chemie (DE-588)4121505-9 gnd rswk-swf Carbon dioxide molecular orbitals CO2 spectroscopic techniques CO2 enzymatic conversion CO2 coordination to metal centres CO2 insertion into 11-X CO2 electrochemical reduction CO2 photocatalytic reduction Chemie/Organische Chemie Kohlendioxid (DE-588)4031648-8 s Ausgangsmaterial (DE-588)4143518-7 s Präparative organische Chemie (DE-588)4121505-9 s Reaktivität (DE-588)4208182-8 s Reaktionsmechanismus (DE-588)4177123-0 s DE-604 Dibenedetto, Angela 1968- Verfasser (DE-588)1043471332 aut Quaranta, Eugenio 1957- Verfasser (DE-588)1142397882 aut Erscheint auch als Online-Ausgabe 978-3-662-46831-9 B:DE-101 application/pdf http://d-nb.info/1068076755/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028864143&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Aresta, Michele 1940- Dibenedetto, Angela 1968- Quaranta, Eugenio 1957- Reaction mechanisms in carbon dioxide conversion Reaktivität (DE-588)4208182-8 gnd Kohlendioxid (DE-588)4031648-8 gnd Reaktionsmechanismus (DE-588)4177123-0 gnd Ausgangsmaterial (DE-588)4143518-7 gnd Präparative organische Chemie (DE-588)4121505-9 gnd |
| subject_GND | (DE-588)4208182-8 (DE-588)4031648-8 (DE-588)4177123-0 (DE-588)4143518-7 (DE-588)4121505-9 |
| title | Reaction mechanisms in carbon dioxide conversion |
| title_auth | Reaction mechanisms in carbon dioxide conversion |
| title_exact_search | Reaction mechanisms in carbon dioxide conversion |
| title_full | Reaction mechanisms in carbon dioxide conversion Michele Aresta, Angela Dibenedetto, Eugenio Quaranta |
| title_fullStr | Reaction mechanisms in carbon dioxide conversion Michele Aresta, Angela Dibenedetto, Eugenio Quaranta |
| title_full_unstemmed | Reaction mechanisms in carbon dioxide conversion Michele Aresta, Angela Dibenedetto, Eugenio Quaranta |
| title_short | Reaction mechanisms in carbon dioxide conversion |
| title_sort | reaction mechanisms in carbon dioxide conversion |
| topic | Reaktivität (DE-588)4208182-8 gnd Kohlendioxid (DE-588)4031648-8 gnd Reaktionsmechanismus (DE-588)4177123-0 gnd Ausgangsmaterial (DE-588)4143518-7 gnd Präparative organische Chemie (DE-588)4121505-9 gnd |
| topic_facet | Reaktivität Kohlendioxid Reaktionsmechanismus Ausgangsmaterial Präparative organische Chemie |
| url | http://d-nb.info/1068076755/04 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028864143&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT arestamichele reactionmechanismsincarbondioxideconversion AT dibenedettoangela reactionmechanismsincarbondioxideconversion AT quarantaeugenio reactionmechanismsincarbondioxideconversion |
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