Interfacial supramolecular assemblies:
Gespeichert in:
| Hauptverfasser: | , , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Chichester
Wiley
2003
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XI, 317 S. graph. Darst. |
| ISBN: | 0471490717 |
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Datensatz im Suchindex
| _version_ | 1804129403364442112 |
|---|---|
| adam_text | INTERFACIAL SUPRAMOLECULAR ASSEMBUES JOHANNES G. VOS ROBERT J. FORSTER
DUBLIN UNIVERSITY, IRELAND TIA E. KEYES DUBLIN INSTITUTE OF TECHNOLOGY,
IRELAND JOHN WILEY & SONS, LTD CONTENTS 1 INTRODUCTION 1 1.1
INTRODUCTORY REMARKS L 1.2 INTERFACIAL SUPRAMOLECULAR CHEMISTRY 2 1.3
OBJECTIVESOFTHIS BOOK 4 1.4 TESTING CONTEMPORARY THEORY USING ISAS 4 1.5
ANALYSIS OF STRUCTURE AND PROPERTIES 5 1.6 FORMATION AND
CHARACTERIZATION OF INTERFACIAL SUPRAMOLECULAR ASSEMBLIES 5 1.7 ELECTRON
AND ENERGY TRANSFER PROPERTIES 6 1.8 INTERFACIAL ELECTRON TRANSFER
PROCESSES AT MODIFIED SEMICONDUCTOR SURFACES 6 FURTHER READING 6 2
THEORETICAL FRAMEWORK FOR ELECTROCHEMICAL AND OPTICAL PROCESSES 9 2.1
INTRODUCTION 9 2.2 ELECTRON TRANSFER 9 2.2.1 HOMOGENOUS ELECTRON
TRANSFER 10 2.2.2 HETEROGENEOUS ELECTRON TRANSFER 21 VI CONTENTS 2.3
PHOTOINDUCED PROCESSES 28 2.3.1 PHOTOCHEMISTRY AND PHOTOPHYSICS OF
SUPRAMOLECULAR MATERIALS 28 2.3.2 PHOTOINDUCED ELECTRON TRANSFER 31
2.3.3 PHOTOINDUCED ENERGY TRANSFER 33 2.3.4 PHOTOINDUCED MOLECULAR
REARRANGEMENTS 36 2.4 PHOTOINDUCED INTERFACIAL ELECTRON TRANSFER 41
2.4.1 DYE-SENSITIZED PHOTOINDUCED ELECTRON TRANSFER AT METAL SURFACES 43
2.4.2 DYE-SENSITIZED PHOTOINDUCED ELECTRON TRANSFER AT SEMICONDUCTOR
SURFACES 44 2.4.3 PHOTOINDUCED INTERFACIAL ENERGY TRANSFER 45 2.5
ELUCIDATION OF EXCITED-STATE MECHANISMS 46 2.0 CONCLUSIONS 48 REFERENCES
AND NOTES 48 5 METHODSOF ANALYSIS 51 3.1 STRUCTURAL CHARACTERIZATION OF
INTERFACIAL SUPRAMOLECULAR ASSEM BLIES 51 3.1.1 SCANNING PROBE
MICROSCOPY 52 3.1.2 SCANNING ELECTROCHEMICAL MICROSCOPY 53 3.1.3 CONTACT
ANGLE MEASUREMENTS 55 3.1.4 MASS-SENSITIVE APPROACHES 56 3.1.5
ELLIPSOMETRY 59 3.1.6 SURFACE PLASMON RESONANCE 60 3.1.7 NEUTRON
REFLECTIVITY 62 3.2 VOLTAMMETRIC PROPERTIES OF INTERFACIAL
SUPRAMOLECULAR ASSEM BLIES 63 3.2.1 ELECTROCHEMICAL PROPERTIES OF AN
IDEAL REDOX-ACTIVE ASSEMBLY 63 3.2.2 THE FORMAL POTENTIAL 66 3.2.3
EFFECT OF LATERAL INTERACTIONS 66 3.2.4 DIFFUSIONAL CHARGE TRANSPORT
THROUGH THIN FILMS 67 3.2.5 ROTATING DISK VOLTAMMETRY 68 3.2.6
INTERFACIAL CAPACITANCE AND RESISTANCE 70 3*3 SPECTROSCOPIC PROPERTIES
OF INTERFACIAL SUPRAMOLECULAR ASSEMBLIES 70 3.3.1 LUMINESCENCE
SPECTROSCOPY 71 3.3.2 FLUORESCENCE DEPOLARIZATION 72 3.3.3
EPIFLUORESCENT AND CONFOCAL MICROSCOPY 73 CONTENTS 3.3.4 NEAR-FIELD
SCANNING OPTICAL MICROSCOPY 3.3.5 RAMAN SPECTROSCOPY 3.3.6 SECOND
HARMONIE GENERATION 3.3.7 SINGLE-MOLECULE SPECTROSCOPY 3.3.8
SPECTROELECTROCHEMISTRY 3.3.9 INTENSITY-MODULATED PHOTOCURRENT
SPECTROSCOPY 3*4 TIME-RESOLVED SPECTROSCOPY OF INTERFACIAL
SUPRAMOLECUIAR ASSEMBLIES 3.4.1 FLASH PHOTOLYSIS 3.4.2 TIME-RESOLVED
LUMINESCENCE TECHNIQUES 3.4.3 FEMTOCHEMISTRY 3*5 CONCLUSIONS REFERENCES
L FORMATION AND CHARACTERIZATION OF MODIFIED SURFACES 4*1 INTRODUCTION
4*2 SUBSTRATE CHOICE AND PREPARATION 4*3 FORMATION OF SELF-ASSEMBLED
MONOLAYERS 4.3.1 SOLUTION-PHASE DEPOSITION 4.3.2 ELECTROCHEMICAL
STRIPPING AND DEPOSITION 4.3.3 THERMODYNAMICS OF ADSORPTION 4.3.4
DOUBLE-LAYER STRUCTURE 4.3.5 POST-DEPOSITION MODIFICATION 4*4 STRUCTURAL
CHARACTERIZATION OF MONOLAYERS 4.4.1 PACKING AND ADSORBATE ORIENTATION
4.4.2 SURFACE PROPERTIES 4*5 ELECTROCHEMICAL CHARACTERIZATION 4.5.1
GENERAL VOLTAMMETRIC PROPERTIES OF REDOX-ACTIVE MONOLAY 4.5.2 MEASURING
THE DEFECT DENSITY 4*6 MULTILAYER FORMATION 4.6.1 ELECTROSTATICALLY
DRIVEN ASSEMBLIES 4.6.2 ORDERED PROTEIN LAYERS 4.6.3 SURFACTANT-BASED
MULTILAYER ASSEMBLIES VIII CONTENTS 4.7 POLYMER FILMS 117 4.7.1 FILM
DEPOSITION METHODS 118 4.7.2 SYNTHETIC PROCEDURES FOR THE PREPARATION OF
REDOX-ACTIVE POLYMERS 121 4.7.3 SYNTHETIC METHODS FOR THE PREPARATION OF
CONDUCTING POLYMERS 126 4*8 STRUCTURAL FEATURES AND STRUCTURE-PROPERTY
RELATIONSHIPS OF THIN POLYMER FILMS 134 4.8.1 STRUCTURAL ASSESSMENT OF
REDOX POLYMERS USING NEUTRON REFLECTIVITY 134 4.8.2 STRUCTURAL FEATURES
OF ELECTROSTATICALLY DEPOSITED MULTILAYER ASSEMBLIES 138 4.8.3
SELF-ASSEMBLED MONOLAYER FILMS OF THIOL-DERIVATIZED POLYMERS 140 4.8.4
STRUCTURAL PROPERTIES OF BLOCK COPOLYMERS 141 4.8.5 DOMAIN CONTROL WITH
STYRENE-METHYL METHACRYLATE COPOLYMERS 143 4.8.6 STRUCTURE-CONDUCTIVITY
RELATIONSHIPS FOR ALKYLTHIOPHENES 144 4*9 BIOMIMETIC ASSEMBLIES 146
4.9.1 PROTEIN LAYERS 147 4.9.2 BIOMOLECULE BINDING TO SELF-ASSEMBLED
MONOLAYERS 148 4.9.3 REDOX PROPERTIES OF BIOMONOLAYERS 149 4.10
CONCLUSIONS 150 REFERENCES 151 ELECTRON AND ENERGY TRANSFER DYNAMICS 153
5*1 INTRODUCTION 153 5*2 ELECTRON AND ENERGY TRANSFER DYNAMICS OF
ADSORBED MONOLAYERS 154 5.2.1 DISTANCE DEPENDENCE OF ELECTRON TRANSFER
155 5.2.2 RESONANCE EFFECTS ON ELECTRON TRANSFER 157 5.2.3 ELECTRODE
MATERIAL EFFECTS ON ELECTRON TRANSFER 162 5.2.4 EFFECT OF BRIDGE
CONJUGATION ON ELECTRON TRANSFER DYNAMICS 165 5.2.5 REDOX PROPERTIES OF
DIMERIC MONOLAYERS 167 5.2.6 COUPLED PROTON AND ELECTRON TRANSFERS IN
MONOLAYERS 169 5.2.7 REDOX-SWITCHABLE LATERAL INTERACTIONS 174 5.2.8
ELECTRON TRANSFER DYNAMICS OF ELECTRONICALLY EXCITED STATES 177 5.2.9
CONFORMATIONAL GATING IN MONOLAYERS 180 5.2.10 ELECTRON TRANSFER WITHIN
BIOSYSTEMS 183 5.2.11 PROTEIN-MEDIATED ELECTRON TRANSFER 183 CONTENTS IX
5*3 NANOPARTICLES AND SELF-ASSEMBLED MONOLAYERS 185 5.3.1 CONDUCTIVITIES
OF SINGLE CLUSTERS - MOLECULAR SWITCHING 186 5*4 ELECTROANALYTICAL
APPLICATIONS 187 5.4.1 MICROARRAY ELECTRODES 187 5.4.2 SELECTIVE
PERMEATION 188 5.4.3 PRECONCENTRATION AND SELECTIVE BINDING 188 5.4.4
SAM-BASED BIOSENSORS 189 5.4.5 KINETIC SEPARATION OF AMPEROMETRIC SENSOR
RESPONSES 190 5*5 LIGHT-ADDRESSABLEASSEMBLIES 192 5*6
SURFACE-PHOTOACTIVE SUBSTRATE INTERACTIONS 193 5*7 PHOTOACTIVE
SELF-ASSEMBLED MONOLAYERS 194 5*8 PHOTOCURRENT GENERATION AT MODIFIED
METAL ELECTRODES 194 5*9 PHOTOINDUCED MOLECULAR SWITCHING 199 5.10
LUMINESCENT FILMS 206 5*11 PHOTOINDUCED PROCESSES IN BIO-SAMS 211 5.12
PHOTOINDUCED ELECTRON AND ENERGY TRANSFER IN SAMS 215 5.12.1 DISTANCE
DEPENDENCE OF PHOTOINDUCED ELECTRON AND ENERGY TRANSFER 216 5.12.2
PHOTOINDUCED ENERGY TRANSFER 219 5.12.3 MONOLAYER MOBILITY AND SUBSTRATE
ROUGHNESS 220 5.13 MULTILAYERASSEMBLIES 223 5.13.1 PHOTOINDUCED CHARGE
SEPARATION IN MULTILAYERS 229 5*14 ELECTROCHEMISTRY OF THIN REDOX-ACTIVE
POLYMER FILMS 235 5.14.1 HOMOGENEOUS CHARGE TRANSPORT 236 5.14.2
ELECTROCHEMICAL QUARTZ CRYSTAL MICROBALANCE STUDIES 239 5.14.3
INTERFACIAL ELECTROCATALYSIS 240 5*15 CONCLUSIONS AND FUTURE DIRECTIONS
247 5.15.1 CHALLENGES FOR THE NEXT DECADE 248 REFERENCES 249 CONTENTS 6
INTERFACIAL ELECTRON TRANSFER PROCESSES AT MODIFIED SEMICONDUCTOR
SURFACES 253 6.1 INTRODUCTION 253 6.2 STRUCTURAL AND ELECTRONIC FEATURES
OF NANOCRYSTALLINE TI0 2 SURFACES 254 6.2.1 ELECTRONIC PROPERTIES OF
BULK TI0 2 254 6.2.2 ELECTRONIC PROPERTIES OF NANOPARTICLES 256 6.2.3
PREPARATION AND STRUCTURAL FEATURES OF NANOCRYSTALLINE TI0 2 SURFACES
259 6.3 PHYSICAL AND CHEMICAL PROPERTIES OF MOLECULAR COMPONENTS 262
6.3.1 CHARGE SEPARATION AT NANOCRYSTALLINE TIC 2 SURFACES 267 6.4
PHOTOVOLTAIC CELLS BASED ON DYE-SENSITIZED TI0 2 269 6.5 PHOTOINDUCED
CHARGE INJECTION 273 6.5.1 EXTERNAL FACTORS WHICH AFFECT PHOTOINDUCED
CHARGE INJECTION 275 6.5.2 COMPOSITION OF ELECTROLYTE 275 6.5.3 THE
EFFECT OF REDOX POTENTIAL 279 6.6 INTERFACIAL SUPRAMOLECULAR ASSEMBLIES
280 6.6.1 RUTHENIUM PHENOTHIAZINE ASSEMBLY 280 6.6.2 RHODIUM-RUTHENIUM
ASSEMBLY 282 6.6.3 RUTHENIUM OSMIUM ASSEMBLY 286 6.7 ELECTROCHEMICAL
BEHAVIOR OF NANOCRYSTALLINE TI0 2 SURFACES 291 6.7.1 ELECTROCHROMIC
DEVICES 294 6.8 ALTERNATIVE SEMICONDUCTOR SUBSTRATES 297 6.9 CONCLUDING
REMARKS 299 REFERENCES 300 301 I CONCLUSIONS AND FUTURE DIRECTIONS 7.1
CONCLUSIONS - WHERE TO FROM HERE ? 301 7.2 MOLECULAR SELF-ASSEMBLY 301
CONTENTS XI 7*3 MOLECULAR COMPONENTS AND NANOTECHNOLOGY 302 7.4
BIOSYSTEMS 303 7.5 SMART PLASTICS* 304 7-6 INTERFACIAL PHOTOCHEMISTRY
AT CONDUCTING SURFACES 305 J.J MODIFIED SEMICONDUCTOR SURFACES 306 7.8
CONCLUDING REMARKS 306 INDEX 309
|
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| illustrated | Illustrated |
| indexdate | 2024-07-09T19:04:35Z |
| institution | BVB |
| isbn | 0471490717 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-009941498 |
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| physical | XI, 317 S. graph. Darst. |
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| publisher | Wiley |
| record_format | marc |
| spelling | Vos, Johannes G. Verfasser aut Interfacial supramolecular assemblies Johannes G. Vos ; Robert J. Forster ; Tia E. Keyes Chichester Wiley 2003 XI, 317 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Biosensoren gtt Elektronenoverdracht gtt Grensvlakchemie gtt Halfgeleiders gtt Optische eigenschappen gtt Polymeren gtt Structuur-activiteit-relatie gtt Supramoleculaire systemen gtt Supramolecular chemistry Surface chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd rswk-swf Supramolekulare Struktur (DE-588)4208977-3 gnd rswk-swf Grenzfläche (DE-588)4021991-4 gnd rswk-swf Supramolekulare Struktur (DE-588)4208977-3 s Grenzfläche (DE-588)4021991-4 s DE-604 Supramolekulare Chemie (DE-588)4306141-2 s Forster, Robert J. Verfasser aut Keyes, Tia E. Verfasser aut GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009941498&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Vos, Johannes G. Forster, Robert J. Keyes, Tia E. Interfacial supramolecular assemblies Biosensoren gtt Elektronenoverdracht gtt Grensvlakchemie gtt Halfgeleiders gtt Optische eigenschappen gtt Polymeren gtt Structuur-activiteit-relatie gtt Supramoleculaire systemen gtt Supramolecular chemistry Surface chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd Supramolekulare Struktur (DE-588)4208977-3 gnd Grenzfläche (DE-588)4021991-4 gnd |
| subject_GND | (DE-588)4306141-2 (DE-588)4208977-3 (DE-588)4021991-4 |
| title | Interfacial supramolecular assemblies |
| title_auth | Interfacial supramolecular assemblies |
| title_exact_search | Interfacial supramolecular assemblies |
| title_full | Interfacial supramolecular assemblies Johannes G. Vos ; Robert J. Forster ; Tia E. Keyes |
| title_fullStr | Interfacial supramolecular assemblies Johannes G. Vos ; Robert J. Forster ; Tia E. Keyes |
| title_full_unstemmed | Interfacial supramolecular assemblies Johannes G. Vos ; Robert J. Forster ; Tia E. Keyes |
| title_short | Interfacial supramolecular assemblies |
| title_sort | interfacial supramolecular assemblies |
| topic | Biosensoren gtt Elektronenoverdracht gtt Grensvlakchemie gtt Halfgeleiders gtt Optische eigenschappen gtt Polymeren gtt Structuur-activiteit-relatie gtt Supramoleculaire systemen gtt Supramolecular chemistry Surface chemistry Supramolekulare Chemie (DE-588)4306141-2 gnd Supramolekulare Struktur (DE-588)4208977-3 gnd Grenzfläche (DE-588)4021991-4 gnd |
| topic_facet | Biosensoren Elektronenoverdracht Grensvlakchemie Halfgeleiders Optische eigenschappen Polymeren Structuur-activiteit-relatie Supramoleculaire systemen Supramolecular chemistry Surface chemistry Supramolekulare Chemie Supramolekulare Struktur Grenzfläche |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009941498&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT vosjohannesg interfacialsupramolecularassemblies AT forsterrobertj interfacialsupramolecularassemblies AT keyestiae interfacialsupramolecularassemblies |